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that TDDFT studies [65, 66] of even standard 3d transition metal ferromagnets\u2014such as Fe, Co, and Ni\u2014have recently started to explore additional effects on ultrafast demagnetization due to Coulomb correlations among the localized d electrons included via the Hubbard 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of interfacial bands often found in DFT calculations [19, 48] displays remarkable similarities [19] to the much simpler Rashba SOC model [Eq.\u00a0(5)]. Although overlap of interfacial orbitals plays an important role in DFT calculations\u2014generating effects [19] like correlation between the spin-splitting strength of the bands and the SOC-weighted induced orbital momentum, as well as orbital charge transfer\u2014we do not model it explicitly by adding a second NM layer with its own orbitals (aside from two selected orbitals per site of NiO layer in Fig.\u00a02 that we model explicitly) due to high computational expense of our quantum many-body calculations (when compared to effective single-body calculations of DFT). Nevertheless, the essential outcome of such complex interfacial processes is included in our Hamiltonian through the Rashba SOC term [Eq.\u00a0(5)], i.e., as k-asymmetric spin splitting [Fig.\u00a01]. Most importantly, our finding that THz emission is significant only when the Rashba SOC is turned on, as well as that in experiments the highest intensity of THz radiation comes from the thinnest NiO layer, is fully compatible with findings of recent experiments [17, 18] on subgap-fsLP-excited NiO\/HM bilayers.","type":"other"},{"key":"8dhn-dh55Cc72R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevLett.93.076401","type":"journal-article"},{"key":"8dhn-dh55Cc73R1","doi-asserted-by":"publisher","DOI":"10.1088\/1742-5468\/2004\/04\/P04005","type":"journal-article"},{"key":"8dhn-dh55Cc74R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.70.121302","type":"journal-article"},{"key":"8dhn-dh55Cc75R1","doi-asserted-by":"publisher","DOI":"10.1063\/1.3667323","type":"journal-article"},{"key":"8dhn-dh55Cc76R1","doi-asserted-by":"publisher","DOI":"10.1140\/epjp\/s13360-020-00919-2","type":"journal-article"},{"key":"8dhn-dh55Cc77R1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cpc.2024.109093","type":"journal-article"},{"key":"8dhn-dh55Cc78R1","doi-asserted-by":"publisher","DOI":"10.1016\/j.cpc.2017.04.006","type":"journal-article"},{"key":"8dhn-dh55Cc79R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevLett.124.137701","type":"journal-article"},{"key":"8dhn-dh55Cc80R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.107.L060305","type":"journal-article"},{"key":"8dhn-dh55Cc81R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevLett.126.197202","type":"journal-article"},{"key":"8dhn-dh55Cc82R1","doi-asserted-by":"publisher","DOI":"10.1080\/00018730701619647","type":"journal-article"},{"key":"8dhn-dh55Cc83R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.75.165115","type":"journal-article"},{"key":"8dhn-dh55Cc84R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.100.035104","type":"journal-article"},{"key":"8dhn-dh55Cc85R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.97.235104","type":"journal-article"},{"key":"8dhn-dh55Cc86R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.103.224434","type":"journal-article"},{"key":"8dhn-dh55Cc87R1","doi-asserted-by":"publisher","DOI":"10.1002\/qute.202400196","type":"journal-article"},{"key":"8dhn-dh55Cc88R1","doi-asserted-by":"publisher","DOI":"10.1007\/s00220-003-0950-1","type":"journal-article"},{"key":"8dhn-dh55Cc89R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.101.205140","type":"journal-article"},{"key":"8dhn-dh55Cc90R1","unstructured":"We have verified that our results are largely insensitive to the inclusion of additional terms required for multiorbital systems [4, 91], such as E(t)\u00b7P(t), where E(t)=\u2212\u2202tA is the electric field of fsLP and P(t) describes the dipolar matrix elements between different orbitals residing on the same site of the lattice.","type":"other"},{"key":"8dhn-dh55Cc91R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.101.035203","type":"journal-article"},{"key":"8dhn-dh55Cc92R1","unstructured":"This is the largest lattice size, hosting two orbitals per site, that we could simulate within a reasonable computational time. For example, the storage cost of the sparse Hamiltonian matrix alone defined for this lattice exceeds 600\u00a0GB. Nevertheless, using such a small ladder is already sufficient to capture various dissipative mechanisms, even in the absence of phonons that are considered necessary for relaxation [57, 93] after weakly correlated magnets are excited by fsLP. For example, in quasi-1D ladder geometry [94, 95], and with more than one orbital per site [85], spin-charge separation characterizing 1D Mott insulators [96, 97] is suppressed. This opens [85, 94] dissipation channels due to electron-spin interaction, where energy is transferred from the electrons to the AFM background [2, 4, 95], as well as local dissipation caused by the Hund interaction [85, 98, 99]. The outcome is that photoexcited charge current decays, even though phonons are absent, as shown in the Supplemental Material [100].","type":"other"},{"key":"8dhn-dh55Cc93R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.107.174421","type":"journal-article"},{"key":"8dhn-dh55Cc94R1","doi-asserted-by":"publisher","DOI":"10.1038\/srep21235","type":"journal-article"},{"key":"8dhn-dh55Cc95R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.89.165118","type":"journal-article"},{"key":"8dhn-dh55Cc96R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevLett.134.096504","type":"journal-article"},{"key":"8dhn-dh55Cc97R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevLett.130.106501","type":"journal-article"},{"key":"8dhn-dh55Cc98R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.101.195139","type":"journal-article"},{"key":"8dhn-dh55Cc99R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevB.96.165104","type":"journal-article"},{"key":"8dhn-dh55Cc100R1","unstructured":"See Supplemental Material at http:\/\/link.aps.org\/supplemental\/10.1103\/8dhn-dh55 for an additional figure showing how the sum of all bond charge currents decays with increasing on-site Coulomb interaction due to thereby enabled dissipation of electron energy into bosonic excitations of AFM ordered background [2,94,95].","type":"other"},{"key":"8dhn-dh55Cc101R1","doi-asserted-by":"publisher","DOI":"10.1038\/nphoton.2010.259","type":"journal-article"},{"key":"8dhn-dh55Cc102R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevLett.105.077402","type":"journal-article"},{"key":"8dhn-dh55Cc103R1","doi-asserted-by":"publisher","DOI":"10.1038\/nphys1369","type":"journal-article"},{"key":"8dhn-dh55Cc104R1","doi-asserted-by":"publisher","DOI":"10.1103\/PhysRevLett.131.096701","type":"journal-article"},{"key":"8dhn-dh55Cc105R1","first-page":"153","type":"journal-article","volume":"8","author":"L.\u2009D. 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