{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,9,9]],"date-time":"2026-09-09T00:36:31Z","timestamp":1788914191261,"version":"build-2803163510"},"reference-count":43,"publisher":"American Association for the Advancement of Science (AAAS)","issue":"47","content-domain":{"domain":["www.science.org"],"crossmark-restriction":true},"short-container-title":["Sci. Adv."],"published-print":{"date-parts":[[2024,11,22]]},"abstract":"<jats:p>\n            To date, the understanding of various modes of CO\n            <jats:sub>2<\/jats:sub>\n            mass transport remains incomplete, impeding the transfer of catalysts identified in the more accessible electrochemical batch cells to high-performance flow cells. In this work, we demonstrate that the meniscus region formed between the electrode and the convex liquid level due to the electrowetting of the catalyst plays a vital role in the CO\n            <jats:sub>2<\/jats:sub>\n            RR in batch cells. CO\n            <jats:sub>2<\/jats:sub>\n            RR in the meniscus region in batch cells exhibits similar performance with that in flow cells, and the performance disparity between these two configurations largely disappears when conducting CO\n            <jats:sub>2<\/jats:sub>\n            RR primarily in the meniscus region. An assembled double-sided gas diffusion electrode with a gas channel is developed to maximize the meniscus-like region, achieving a CO\n            <jats:sub>2<\/jats:sub>\n            RR partial current density of 640 mA\/cm\n            <jats:sup>2<\/jats:sup>\n            <jats:sub>geo<\/jats:sub>\n            on commercial Cu in the KHCO\n            <jats:sub>3<\/jats:sub>\n            electrolyte. This performance represents the highest CO\n            <jats:sub>2<\/jats:sub>\n            RR activity in neutral buffered media.\n          <\/jats:p>","DOI":"10.1126\/sciadv.adp5697","type":"journal-article","created":{"date-parts":[[2024,11,22]],"date-time":"2024-11-22T19:10:42Z","timestamp":1732302642000},"update-policy":"https:\/\/doi.org\/10.34133\/aaas_crossmark","source":"Crossref","is-referenced-by-count":23,"title":["Bridging activity gaps between batch and flow reactor configurations in the electroreduction of carbon dioxide"],"prefix":"10.1126","volume":"10","author":[{"ORCID":"https:\/\/orcid.org\/0009-0002-3101-6462","authenticated-orcid":true,"given":"Qiwen","family":"Sun","sequence":"first","affiliation":[{"name":"College of Chemistry and Molecular Engineering, Peking University, Beijing 100871, China."}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-6733-9031","authenticated-orcid":true,"given":"Linke","family":"Fu","sequence":"additional","affiliation":[{"name":"College of Chemistry and Molecular Engineering, Peking University, Beijing 100871, China."}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-6598-6083","authenticated-orcid":true,"given":"Xiaoxia","family":"Chang","sequence":"additional","affiliation":[{"name":"College of Chemistry and Molecular Engineering, Peking University, Beijing 100871, China."}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-2303-257X","authenticated-orcid":true,"given":"Bingjun","family":"Xu","sequence":"additional","affiliation":[{"name":"College of Chemistry and Molecular Engineering, Peking University, Beijing 100871, China."}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"221","reference":[{"key":"e_1_3_2_2_2","doi-asserted-by":"publisher","DOI":"10.1016\/0013-4686(94)85172-7"},{"key":"e_1_3_2_3_2","doi-asserted-by":"publisher","DOI":"10.3866\/PKU.WHXB202206020"},{"key":"e_1_3_2_4_2","doi-asserted-by":"publisher","DOI":"10.1038\/s44286-024-00076-8"},{"key":"e_1_3_2_5_2","doi-asserted-by":"publisher","DOI":"10.1039\/C8EE00097B"},{"key":"e_1_3_2_6_2","doi-asserted-by":"publisher","DOI":"10.1021\/acs.iecr.1c03592"},{"key":"e_1_3_2_7_2","doi-asserted-by":"publisher","DOI":"10.1021\/acs.chemrev.8b00705"},{"key":"e_1_3_2_8_2","doi-asserted-by":"publisher","DOI":"10.1088\/2515-7655\/ac7823"},{"key":"e_1_3_2_9_2","doi-asserted-by":"publisher","DOI":"10.1021\/jacsau.3c00494"},{"key":"e_1_3_2_10_2","doi-asserted-by":"publisher","DOI":"10.1149\/1.2044182"},{"key":"e_1_3_2_11_2","doi-asserted-by":"publisher","DOI":"10.1038\/s41929-018-0133-2"},{"key":"e_1_3_2_12_2","doi-asserted-by":"publisher","DOI":"10.1126\/science.aas9100"},{"key":"e_1_3_2_13_2","doi-asserted-by":"publisher","DOI":"10.1016\/j.joule.2021.02.008"},{"key":"e_1_3_2_14_2","doi-asserted-by":"publisher","DOI":"10.3866\/PKU.WHXB202302037"},{"key":"e_1_3_2_15_2","doi-asserted-by":"publisher","DOI":"10.1016\/j.electacta.2018.04.072"},{"key":"e_1_3_2_16_2","doi-asserted-by":"publisher","DOI":"10.1021\/jacs.0c13427"},{"key":"e_1_3_2_17_2","doi-asserted-by":"publisher","DOI":"10.1016\/j.joule.2020.03.013"},{"key":"e_1_3_2_18_2","doi-asserted-by":"publisher","DOI":"10.1039\/D1EE01696B"},{"key":"e_1_3_2_19_2","doi-asserted-by":"publisher","DOI":"10.1021\/acsenergylett.2c00763"},{"key":"e_1_3_2_20_2","doi-asserted-by":"publisher","DOI":"10.1021\/jacs.9b11817"},{"key":"e_1_3_2_21_2","doi-asserted-by":"publisher","DOI":"10.1021\/jacs.2c09378"},{"key":"e_1_3_2_22_2","doi-asserted-by":"publisher","DOI":"10.1038\/s41929-022-00776-5"},{"key":"e_1_3_2_23_2","doi-asserted-by":"publisher","DOI":"10.1039\/D3CC00705G"},{"key":"e_1_3_2_24_2","doi-asserted-by":"publisher","DOI":"10.1021\/acscatal.0c03319"},{"key":"e_1_3_2_25_2","doi-asserted-by":"publisher","DOI":"10.1021\/acscatal.9b00099"},{"key":"e_1_3_2_26_2","doi-asserted-by":"publisher","DOI":"10.1002\/anie.202315822"},{"key":"e_1_3_2_27_2","doi-asserted-by":"publisher","DOI":"10.1038\/s41467-021-23582-2"},{"key":"e_1_3_2_28_2","doi-asserted-by":"publisher","DOI":"10.1088\/0953-8984\/17\/28\/R01"},{"key":"e_1_3_2_29_2","doi-asserted-by":"publisher","DOI":"10.1063\/1.1671193"},{"key":"e_1_3_2_30_2","first-page":"9735","article-title":"Speciation of Cu surfaces during the electrochemical CO reduction reaction","volume":"142","author":"Zhao Y.","year":"2020","unstructured":"Y. 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