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Similar findings to the Urey-Miller experiment were observed by spraying room temperature water microdroplets into a gas mixture containing nitrogen, methane, carbon dioxide, and ammonia, which leads to the synthesis of organic molecules containing carbon-nitrogen (C\u2500N) bonds. These observations provide another explanation for unique reactivity at the gas-water interface, as well as a possible mechanism for making the building blocks of life on early Earth.<\/jats:p>","DOI":"10.1126\/sciadv.adt8979","type":"journal-article","created":{"date-parts":[[2025,3,14]],"date-time":"2025-03-14T13:58:26Z","timestamp":1741960706000},"update-policy":"https:\/\/doi.org\/10.34133\/aaas_crossmark","source":"Crossref","is-referenced-by-count":96,"title":["Spraying of water microdroplets forms luminescence and causes chemical reactions in surrounding gas"],"prefix":"10.1126","volume":"11","author":[{"ORCID":"https:\/\/orcid.org\/0000-0001-6897-3595","authenticated-orcid":true,"given":"Yifan","family":"Meng","sequence":"first","affiliation":[{"name":"Department of Chemistry, Stanford University, Stanford, CA 94305, USA."}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-7647-4921","authenticated-orcid":true,"given":"Yu","family":"Xia","sequence":"additional","affiliation":[{"name":"Department of Chemistry, Stanford University, Stanford, CA 94305, USA."},{"name":"School of Environment and Health, Jianghan University, Wuhan 430056, China."}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0009-0007-1187-5389","authenticated-orcid":true,"given":"Jinheng","family":"Xu","sequence":"additional","affiliation":[{"name":"Department of Chemistry, Stanford University, Stanford, CA 94305, USA."}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-5266-4253","authenticated-orcid":true,"given":"Richard N.","family":"Zare","sequence":"additional","affiliation":[{"name":"Department of Chemistry, Stanford University, Stanford, CA 94305, USA."}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"221","reference":[{"key":"e_1_3_2_2_2","doi-asserted-by":"publisher","DOI":"10.1098\/rspl.1867.0019"},{"key":"e_1_3_2_3_2","doi-asserted-by":"publisher","DOI":"10.1029\/JD090iD04p06013"},{"key":"e_1_3_2_4_2","doi-asserted-by":"publisher","DOI":"10.1126\/science.148.3674.1179"},{"key":"e_1_3_2_5_2","doi-asserted-by":"publisher","DOI":"10.1021\/jp102719s"},{"key":"e_1_3_2_6_2","doi-asserted-by":"publisher","DOI":"10.1016\/j.mattod.2019.05.016"},{"key":"e_1_3_2_7_2","doi-asserted-by":"publisher","DOI":"10.1021\/acs.chemrev.1c00176"},{"key":"e_1_3_2_8_2","doi-asserted-by":"publisher","DOI":"10.1080\/00018738000101466"},{"key":"e_1_3_2_9_2","doi-asserted-by":"publisher","DOI":"10.1039\/D3CS00763D"},{"key":"e_1_3_2_10_2","doi-asserted-by":"publisher","DOI":"10.1002\/andp.18922820805"},{"key":"e_1_3_2_11_2","doi-asserted-by":"publisher","DOI":"10.1073\/pnas.2307977120"},{"key":"e_1_3_2_12_2","doi-asserted-by":"publisher","DOI":"10.1021\/jp806995h"},{"key":"e_1_3_2_13_2","doi-asserted-by":"publisher","DOI":"10.1021\/acs.jpca.4c02981"},{"key":"e_1_3_2_14_2","doi-asserted-by":"publisher","DOI":"10.1021\/acs.analchem.4c00371"},{"key":"e_1_3_2_15_2","first-page":"451","article-title":"Visible light from clear liquids under the action of gamma radiation","volume":"2","author":"Cherenkov P. 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