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While remarkable progress has been made in catalysts, solution design, and system engineering, recent breakthroughs reveal that nitrogen-containing molecules\u2014specifically sp\n                    <jats:sup>2<\/jats:sup>\n                    -hybridized structures (e.g., pyridine) and sp\n                    <jats:sup>3<\/jats:sup>\n                    -hybridized moieties (e.g., ethanolamine) \u2014hold untapped potential to revolutionize both CO\n                    <jats:sub>2<\/jats:sub>\n                    capture and conversion. These structures have been demonstrated as the Holy Grail in facilitating CO\n                    <jats:sub>2<\/jats:sub>\n                    activation, stabilizing key intermediates, and streamlining reaction pathways\u2014capabilities rarely achievable with conventional strategies. However, limited mechanistic understanding of their physicochemical properties and interactions with CO\n                    <jats:sub>2<\/jats:sub>\n                    hampers broader application. This review highlights recent advances in leveraging sp\n                    <jats:sup>2<\/jats:sup>\n                    \/sp\n                    <jats:sup>3<\/jats:sup>\n                    -hybridized nitrogen structures, unpacks their molecular roles in electrochemical CO\n                    <jats:sub>2<\/jats:sub>\n                    management, and offers a unifying framework for their dual-functionality across capture and conversion. By illuminating these nitrogen-based motifs, we uncover practical design principles and open avenues for integrating expanded N-containing compounds into energy technologies\u2014paving the way for next-generation carbon management strategies.\n                  <\/jats:p>","DOI":"10.1126\/sciadv.adw6592","type":"journal-article","created":{"date-parts":[[2025,6,20]],"date-time":"2025-06-20T13:58:33Z","timestamp":1750427913000},"update-policy":"https:\/\/doi.org\/10.34133\/aaas_crossmark","source":"Crossref","is-referenced-by-count":27,"title":["sp\n                    <sup>2<\/sup>\n                    \/sp\n                    <sup>3<\/sup>\n                    \u2013Hybridized nitrogen\u2013mediated electrochemical CO\n                    <sub>2<\/sub>\n                    capture and 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