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Adv."],"published-print":{"date-parts":[[2026,9,4]]},"abstract":"<jats:p>\n                    Balancing specific energy and cycle durability remains a critical challenge for practical battery systems, as conventional single-mechanism anodes struggle to optimize both simultaneously. Here, we engineer a symbiotic Li-SiO\n                    <jats:italic toggle=\"yes\">\n                      <jats:sub>x<\/jats:sub>\n                    <\/jats:italic>\n                    hybrid anode enabling spatiotemporally coordinated Li metal plating and Li-ion alloying. The preferential lithiated Li\n                    <jats:italic toggle=\"yes\">\n                      <jats:sub>x<\/jats:sub>\n                    <\/jats:italic>\n                    Si forms a Li\n                    <jats:sup>+<\/jats:sup>\n                    -conductive network, guiding and confining lithium nucleation beneath the SiO\n                    <jats:italic toggle=\"yes\">\n                      <jats:sub>x<\/jats:sub>\n                    <\/jats:italic>\n                    layer. This precise control over Li plating replenishes active lithium inventory, stabilizing electrochemical reactions and minimizing Li loss. When paired with a LiNi\n                    <jats:sub>0.8<\/jats:sub>\n                    Co\n                    <jats:sub>0.1<\/jats:sub>\n                    Mn\n                    <jats:sub>0.1<\/jats:sub>\n                    O\n                    <jats:sub>2<\/jats:sub>\n                    cathode (4 milliampere-hours per square centimeter), the full cell achieves 50% higher specific energy than SiO\n                    <jats:italic toggle=\"yes\">\n                      <jats:sub>x<\/jats:sub>\n                    <\/jats:italic>\n                    -based lithium-ion batteries while retaining 80% capacity after 900 cycles at a lean negative\/positive ratio of 1.5, outperforming state-of-the-art Li-ion and Li-metal battery systems. A pouch cell exhibits stable cycling over 600 cycles at 0.5C, validating its practicality. Our findings pioneered a universal hybrid anode design paradigm with coupled reaction mechanisms, effectively addressing the longstanding energy durability trade-off in next-generation batteries.\n                  <\/jats:p>","DOI":"10.1126\/sciadv.aea3247","type":"journal-article","created":{"date-parts":[[2026,9,4]],"date-time":"2026-09-04T17:58:46Z","timestamp":1788544726000},"update-policy":"https:\/\/doi.org\/10.34133\/aaas_crossmark","source":"Crossref","is-referenced-by-count":0,"title":["A Li metal-SiO\n                    <i>\n                      <sub>x<\/sub>\n                    <\/i>\n                    hybrid anode enabling synergistic plating\/alloying dual-mechanism lithium storage"],"prefix":"10.1126","volume":"12","author":[{"ORCID":"https:\/\/orcid.org\/0009-0009-5002-1890","authenticated-orcid":true,"given":"Chao-Hui","family":"Zhang","sequence":"first","affiliation":[{"name":"CAS Key Laboratory of Molecular Nanostructure and Nanotechnology, Beijing National Laboratory for Molecular Sciences (BNLMS), Institute of Chemistry, Chinese Academy of Sciences (CAS), Beijing 100190, P. R. China."}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-1690-5616","authenticated-orcid":true,"given":"Juan","family":"Zhang","sequence":"additional","affiliation":[{"name":"CAS Key Laboratory of Molecular Nanostructure and Nanotechnology, Beijing National Laboratory for Molecular Sciences (BNLMS), Institute of Chemistry, Chinese Academy of Sciences (CAS), Beijing 100190, P. R. China."}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yu-Hao","family":"Wang","sequence":"additional","affiliation":[{"name":"CAS Key Laboratory of Molecular Nanostructure and Nanotechnology, Beijing National Laboratory for Molecular Sciences (BNLMS), Institute of Chemistry, Chinese Academy of Sciences (CAS), Beijing 100190, P. R. China."},{"name":"School of Chemical Sciences, University of Chinese Academy of Sciences, Beijing 100049, P. R. China."}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-6851-4313","authenticated-orcid":true,"given":"Shuang-Jie","family":"Tan","sequence":"additional","affiliation":[{"name":"CAS Key Laboratory of Molecular Nanostructure and Nanotechnology, Beijing National Laboratory for Molecular Sciences (BNLMS), Institute of Chemistry, Chinese Academy of Sciences (CAS), Beijing 100190, P. R. China."}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yu-Jie","family":"Guo","sequence":"additional","affiliation":[{"name":"CAS Key Laboratory of Molecular Nanostructure and Nanotechnology, Beijing National Laboratory for Molecular Sciences (BNLMS), Institute of Chemistry, Chinese Academy of Sciences (CAS), Beijing 100190, P. R. China."},{"name":"School of Chemical Sciences, University of Chinese Academy of Sciences, Beijing 100049, P. R. China."}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jun-Chen","family":"Guo","sequence":"additional","affiliation":[{"name":"CAS Key Laboratory of Molecular Nanostructure and Nanotechnology, Beijing National Laboratory for Molecular Sciences (BNLMS), Institute of Chemistry, Chinese Academy of Sciences (CAS), Beijing 100190, P. R. China."}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xiao-Xi","family":"Luo","sequence":"additional","affiliation":[{"name":"CAS Key Laboratory of Molecular Nanostructure and Nanotechnology, Beijing National Laboratory for Molecular Sciences (BNLMS), Institute of Chemistry, Chinese Academy of Sciences (CAS), Beijing 100190, P. R. China."}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jian-Song","family":"Wu","sequence":"additional","affiliation":[{"name":"CAS Key Laboratory of Molecular Nanostructure and Nanotechnology, Beijing National Laboratory for Molecular Sciences (BNLMS), Institute of Chemistry, Chinese Academy of Sciences (CAS), Beijing 100190, P. R. China."},{"name":"School of Chemical Sciences, University of Chinese Academy of Sciences, Beijing 100049, P. R. China."}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-0546-0626","authenticated-orcid":true,"given":"Sen","family":"Xin","sequence":"additional","affiliation":[{"name":"CAS Key Laboratory of Molecular Nanostructure and Nanotechnology, Beijing National Laboratory for Molecular Sciences (BNLMS), Institute of Chemistry, Chinese Academy of Sciences (CAS), Beijing 100190, P. R. China."},{"name":"School of Chemical Sciences, University of Chinese Academy of Sciences, Beijing 100049, P. 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