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This study introduces a composite membrane based on porous graphene oxide (PGO) with two-dimensional copper 1,4-benzenedicarboxylate (CuBDC) nanosheets grown in situ. The confined growth of CuBDC within the PGO laminar structure, via strong coordination between Cu\n                    <jats:sup>2+<\/jats:sup>\n                    ions and oxygen-containing groups on PGO, not only stabilizes the PGO laminar structure but also induces NaCl rejection due to the appropriate pore size of the CuBDC. The resulting composite membrane demonstrated a high-water flux of 124 kg m\n                    <jats:sup>\u22122<\/jats:sup>\n                    \u00a0hour\n                    <jats:sup>\u22121<\/jats:sup>\n                    in conventional pervaporation and 89 kg m\n                    <jats:sup>\u22122<\/jats:sup>\n                    \u00a0hour\n                    <jats:sup>\u22121<\/jats:sup>\n                    in low-energy water carrier pervaporation, with NaCl rejection consistently above 99.9%. Technoeconomic analysis reveals that desalination using the fabricated membrane in a water-carrier pervaporation process results in a low annual expenditure. 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