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Key findings include the identification of cyclopentyl methyl ether as a \u201cgreen\u201d processing solvent for mild deconstruction and an understanding of the catalytic fragmentation mechanism wherein both ring-closing metathesis and chain transfer pathways are present. The deconstruction protocol is shown to be effective for a variety of pDCPD samples produced via distinct ring-opening metathesis polymerization (ROMP) curing methods, including frontal-ROMP, photoROMP, and thermal ROMP, as well as with commercial thermoset formulations and fiber-reinforced composites. As a proof of concept for future translatability, embedded electronics, glass fibers, pristine carbon fibers, and &gt;90% recovery of polymer fragments are demonstrated. 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