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Adv."],"published-print":{"date-parts":[[2026,9,11]]},"abstract":"\n Ultrafast photoexcitation can drive solids far from equilibrium by dynamically renormalizing their electronic structure, yet direct time-domain access to bulk band-structure reshaping with orbital and momentum selectivity has remained limited. Here, we show in photoexcited graphite that femtosecond carbon\n K<\/jats:italic>\n -edge resonant inelastic x-ray scattering (RIXS), used in the time domain, provides a momentum- and orbital-selective spectroscopic fingerprint of transient valence-band reshaping. Momentum- and orbital-selective measurements along the\n \n \n \n K<\/mml:mi>\n \u2192<\/mml:mo>\n M<\/mml:mi>\n <\/mml:mrow>\n <\/mml:math>\n <\/jats:inline-formula>\n contour disentangle\n \n \n \n \u03c0<\/mml:mi>\n <\/mml:mrow>\n <\/mml:math>\n <\/jats:inline-formula>\n and\n \n \n \n \u03c3<\/mml:mi>\n <\/mml:mrow>\n <\/mml:math>\n <\/jats:inline-formula>\n contributions and reveal a structured redistribution of spectral weight emerging within \u223c70 femtoseconds and evolving on picosecond timescales. Nonequilibrium first-principles RIXS calculations performed within a frozen-lattice approximation show that the earliest response is dominated by electronic correlations and transient screening. At longer delays, the dynamics become strongly momentum dependent: Near\n \n \n \n K<\/mml:mi>\n <\/mml:mrow>\n <\/mml:math>\n <\/jats:inline-formula>\n , the signal reflects the decay of the electronic contribution to the renormalized band structure under a hot-phonon bottleneck, whereas at the\n \n \n \n M<\/mml:mi>\n <\/mml:mrow>\n <\/mml:math>\n <\/jats:inline-formula>\n -point van Hove singularity, it reveals a characteristic spectroscopic signature consistent with electron-phonon\u2013driven band red shift and lifetime broadening induced by strongly coupled optical phonons. A three-temperature model constrained by the orbital-resolved tr-RIXS data captures the ensuing energy cascade through a hot-phonon reservoir dominated by the\n \n \n \n \n E<\/mml:mi>\n \n 2<\/mml:mn>\n g<\/mml:mi>\n <\/mml:mrow>\n <\/mml:msub>\n <\/mml:mrow>\n <\/mml:math>\n <\/jats:inline-formula>\n and\n \n \n \n \n A<\/mml:mi>\n 1<\/mml:mn>\n \u2032<\/mml:mo>\n <\/mml:msubsup>\n <\/mml:mrow>\n <\/mml:math>\n <\/jats:inline-formula>\n modes. These results establish time-domain RIXS as a complementary probe of transient band-structure renormalization and mode-selective energy flow in quantum materials.\n <\/jats:p>","DOI":"10.1126\/sciadv.aeg6983","type":"journal-article","created":{"date-parts":[[2026,9,11]],"date-time":"2026-09-11T17:58:29Z","timestamp":1789149509000},"update-policy":"https:\/\/doi.org\/10.34133\/aaas_crossmark","source":"Crossref","is-referenced-by-count":0,"title":["Ultrafast RIXS of orbital-resolved valence-band reshaping in photoexcited graphite"],"prefix":"10.1126","volume":"12","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-4418-035X","authenticated-orcid":true,"given":"Marco","family":"Malvestuto","sequence":"first","affiliation":[{"name":"Elettra Sincrotrone Trieste, SS. 14, Km 163.5, 34149 Trieste, Italy."},{"name":"CNR-Istituto Officina dei Materiali (IOM), SS. 14, Km 163.5, 34149 Trieste, Italy."}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-0580-3542","authenticated-orcid":true,"given":"Antonio","family":"Caretta","sequence":"additional","affiliation":[{"name":"Elettra Sincrotrone Trieste, SS. 14, Km 163.5, 34149 Trieste, Italy."}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8971-6608","authenticated-orcid":true,"given":"Simone","family":"Laterza","sequence":"additional","affiliation":[{"name":"Elettra Sincrotrone Trieste, SS. 14, Km 163.5, 34149 Trieste, Italy."}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-3927-4239","authenticated-orcid":true,"given":"Richa","family":"Bhardwaj","sequence":"additional","affiliation":[{"name":"Elettra Sincrotrone Trieste, SS. 14, Km 163.5, 34149 Trieste, 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