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Adv."],"published-print":{"date-parts":[[2026,10,2]]},"abstract":"<jats:p>\n                    Simultaneously achieving fast kinetics and interfacial stability remains a formidable challenge for quasi-solid-state zinc-iodine batteries. Herein, we introduce the interfacial kosmotropic effect via a low-cost CaSO\n                    <jats:sub>4<\/jats:sub>\n                    \u00b72H\n                    <jats:sub>2<\/jats:sub>\n                    O ionic matrix to actively reconstruct the interfacial chemistry. Through the precise regulation of the electrical double layer, the strong electrostatic fields from surface-bound kosmotropic ions organize limited water molecules into a low-activity, confined network, fundamentally reshaping the solvation structure. Benefiting from this optimized atomic-level architecture, the reaction pathways are fundamentally altered: on the cathode, it unlocks a single-step I\n                    <jats:sup>\u2212<\/jats:sup>\n                    \/I\n                    <jats:sub>2<\/jats:sub>\n                    redox process that effectively severs the formation pathway of polyiodides; on the anode, it induces coordinatively unsaturated structures to accelerate desolvation and suppress parasitic reactions. Consequently, the system circumvents intrinsic kinetic limitations and facilitates a transition from electric-field-driven electromigration to regulated diffusion-dominated transport. This optimizes ion flux and enables stable Zn anode operation for &gt;1000 h (99.7% avg. Coulombic efficiency). The Zn-I\n                    <jats:sub>2<\/jats:sub>\n                    full cells deliver a high areal capacity of 0.91 mAh cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    with 93% capacity retention after 2500 cycles at 1.0 mA cm\n                    <jats:sup>\u22122<\/jats:sup>\n                    . Impressively, this strategy enables a minimalist iodine-free cathode design and successfully scales to pouch cells (stable for &gt;600 cycles), offering a paradigm shift for developing safe, high-rate and durable quasi-solid-state batteries.\n                  <\/jats:p>","DOI":"10.1126\/sciadv.aeg8302","type":"journal-article","created":{"date-parts":[[2026,10,2]],"date-time":"2026-10-02T17:59:16Z","timestamp":1790963956000},"update-policy":"https:\/\/doi.org\/10.34133\/aaas_crossmark","source":"Crossref","is-referenced-by-count":0,"title":["Harnessing interfacial kosmotropic effect for reversible quasi-solid-state zinc-iodine batteries"],"prefix":"10.1126","volume":"12","author":[{"ORCID":"https:\/\/orcid.org\/0009-0002-7492-0566","authenticated-orcid":true,"given":"Yicai","family":"Pan","sequence":"first","affiliation":[{"name":"Department of Materials Science and Engineering &amp; Center of Super-Diamond and Advanced Films (COSDAF), City University of Hong Kong, Hong Kong SAR 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