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This reaction is enabled by a catalyst containing a high density of atomic Pt\n                    <jats:sub>1<\/jats:sub>\n                    and Ir\n                    <jats:sub>1<\/jats:sub>\n                    species supported on a reactive alpha-molybdenum carbide substrate, achieving a hydrogen production rate of 331.3 millimoles of hydrogen per gram catalyst per hour and an acetic acid selectivity of 84.5% at 270\u00b0C, and is therefore more energy-efficient compared with standard reforming. 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