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We report that a lattice-matched Prussian blue scaffold directs heterogeneous nucleation to produce highly oriented, strain-relaxed films. Its redox-active Fe\u2013C\u2261N\u2013Fe network mediates the conversion of Pb\n                    <jats:sup>0<\/jats:sup>\n                    and I\n                    <jats:sup>0<\/jats:sup>\n                    defects, and its rigid open framework suppresses A-site cation redistribution and the resulting electronic inhomogeneity under bias. This strategy yielded champion power conversion efficiencies of 26.1% (n-i-p) and 26.9% (p-i-n; 26.2% certified), scaling to 23.4% in 6-centimeter\u2013by\u20136-centimeter minimodules and a certified 22.9% in 30-centimeter\u2013by\u201330-centimeter submodules. Submodules with initial power conversion efficiencies ranging from 20.2 to 21.0% showed robust durability under accelerated aging and no discernible decline relative to a silicon reference over 5 months of outdoor testing.\n                  <\/jats:p>","DOI":"10.1126\/science.aef5487","type":"journal-article","created":{"date-parts":[[2026,9,24]],"date-time":"2026-09-24T18:00:41Z","timestamp":1790272841000},"page":"1329-1334","update-policy":"https:\/\/doi.org\/10.34133\/aaas_crossmark","source":"Crossref","is-referenced-by-count":0,"title":["Prussian blue regulates ion dynamics in perovskite solar cells"],"prefix":"10.1126","volume":"393","author":[{"ORCID":"https:\/\/orcid.org\/0009-0004-5095-2584","authenticated-orcid":true,"given":"Fang","family":"Cao","sequence":"first","affiliation":[{"name":"State Key Laboratory of Physical Chemistry of Solid Surfaces, Innovation Laboratory for Sciences and Technologies of Energy Materials of Fujian Province (IKKEM), Collaborative Innovation 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