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This study aims to bridge the gap between diffusion studies in simplified and complex natural systems by investigating the incorporation and mobility of Al in natural rutile and its high-pressure polymorph TiO\n            <jats:sub>2<\/jats:sub>\n            (II).\n          <\/jats:p>\n          <jats:p>\n            Experiments were performed at 0.1 MPa to 7 GPa, 1223\u20131373 K, at buffered \u03bc(Al\n            <jats:sub>2<\/jats:sub>\n            O\n            <jats:sub>3<\/jats:sub>\n            ) and with\n            <jats:italic>f<\/jats:italic>\n            O\n            <jats:sub>2<\/jats:sub>\n            constrained to \u2264CCO, which is the equilibrium between graphite and a CO-CO\n            <jats:sub>2<\/jats:sub>\n            gas phase. Based on electron probe microanalysis, secondary ion mass spectrometry and Fourier transform infrared analyses, we suggest a complex combination of mechanisms to explain the incorporation of Al and H in natural rutile and TiO\n            <jats:sub>2<\/jats:sub>\n            (II). This includes: (1) the incorporation of Al\n            <jats:sup>3+<\/jats:sup>\n            on octahedral Ti-sites charge balanced by the formation of oxygen vacancies; and (2) the incorporation of oxygen in interstitial positions charge balanced by hydrogen interstitials.\n          <\/jats:p>\n          <jats:p>\n            Determined Al-diffusivities in natural TiO\n            <jats:sub>2<\/jats:sub>\n            are approximately eight to nine orders of magnitude faster compared to previously published data. A possible explanation includes a significantly enhanced rate of ionic diffusion through the combined effect of hydrolytic weakening, enhanced Al-diffusion through extended defects and to a minor extent oxygen fugacity variations. Consequently, results of this study question that the inferred high closure temperatures for the Al-in-rutile geothermobarometer can be applied to all natural systems.\n          <\/jats:p>","DOI":"10.1144\/sp537-2022-187","type":"journal-article","created":{"date-parts":[[2023,9,14]],"date-time":"2023-09-14T13:55:15Z","timestamp":1694699715000},"page":"123-147","update-policy":"https:\/\/doi.org\/10.1144\/crossmark-policy","source":"Crossref","is-referenced-by-count":2,"title":["Al and H incorporation and Al-diffusion in natural rutile and its high-pressure polymorph TiO\n            <sub>2<\/sub>\n            (II)"],"prefix":"10.1144","volume":"537","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-2134-004X","authenticated-orcid":false,"given":"Bastian","family":"Joachim-Mrosko","sequence":"first","affiliation":[{"name":"University of Innsbruck, Faculty of Geo- and Atmospheric Sciences, Institute of Mineralogy and Petrography, Innrain 52, 6020 Innsbruck, Austria"}]},{"given":"J\u00fcrgen","family":"Konzett","sequence":"additional","affiliation":[{"name":"University of Innsbruck, Faculty of Geo- and Atmospheric Sciences, Institute of Mineralogy and Petrography, Innrain 52, 6020 Innsbruck, Austria"}]},{"given":"Thomas","family":"Ludwig","sequence":"additional","affiliation":[{"name":"Institute of Earth Sciences, Heidelberg University, Im Neuenheimer Feld 234-236, 69120 Heidelberg, Germany"}]},{"given":"Thomas","family":"Griffiths","sequence":"additional","affiliation":[{"name":"Department of Lithospheric Research, University of Vienna, Josef-Holaubek-Platz 2, 1090 Vienna, Austria"}]},{"given":"Gerlinde","family":"Habler","sequence":"additional","affiliation":[{"name":"Department of Lithospheric Research, University of Vienna, Josef-Holaubek-Platz 2, 1090 Vienna, Austria"}]},{"given":"Eugen","family":"Libowitzky","sequence":"additional","affiliation":[{"name":"Department of Mineralogy and Crystallography, University of Vienna, Josef-Holaubek-Platz 2, 1090 Vienna, Austria"}]},{"given":"Roland","family":"Stalder","sequence":"additional","affiliation":[{"name":"University of Innsbruck, Faculty of Geo- and Atmospheric Sciences, Institute of Mineralogy and Petrography, Innrain 52, 6020 Innsbruck, Austria"}]}],"member":"1881","published-online":{"date-parts":[[2023,10,18]]},"reference":[{"key":"e_1_3_6_2_1","doi-asserted-by":"publisher","DOI":"10.1134\/S1028334X09070253"},{"key":"e_1_3_6_3_1","first-page":"447","article-title":"High-pressure high-temperature stability of \u03b1-PbO2-type TiO2 and MgSiO3 majorite: calorimetric and in situ X-ray diffraction studies","volume":"67","author":"Akaogi M.","year":"1992","unstructured":"Akaogi, M., Kusaba, K. 1992. 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