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Express"],"published-print":{"date-parts":[[2021,2,1]]},"abstract":"<jats:p>We present and model a dark-field illumination scheme for coherent anti-Stokes Raman scattering (DF-CARS) that highlights the interfaces of an object with chemical sensitivity. The proposed DF-CARS scheme uses dedicated arrangements of the pump <jats:bold>k<\/jats:bold><jats:sub><jats:italic>p<\/jats:italic>1<\/jats:sub>, Stokes <jats:bold>k<\/jats:bold><jats:sub>\n      <jats:italic>S<\/jats:italic>\n    <\/jats:sub> and probe <jats:bold>k<\/jats:bold><jats:sub><jats:italic>p<\/jats:italic>2<\/jats:sub> beams\u2019 k-wave-vectors to address the sample\u2019s interfaces along the x, y or z axis. The arrangements of the incident k-wave-vectors are derived from the Ewald sphere representation of the outgoing anti-Stokes radiation and the effective CARS excitation wave-vector <jats:bold>k<\/jats:bold><jats:sub>eff<\/jats:sub>\u2009=\u2009<jats:bold>k<\/jats:bold><jats:sub><jats:italic>p<\/jats:italic>1<\/jats:sub>\u2009+\u2009<jats:bold>k<\/jats:bold><jats:sub><jats:italic>p<\/jats:italic>2<\/jats:sub>\u2009\u2212\u2009<jats:bold>k<\/jats:bold><jats:sub>\n      <jats:italic>S<\/jats:italic>\n    <\/jats:sub> under the intention to avoid probing the object frequency <jats:bold>K<\/jats:bold>(0,0,0), i.e., the contribution of a homogeneous sample (dark-field configuration). We suggest a possible experimental realization using simple masks placed in the back pupil of the excitation microscope objective lens. Applying a full vectorial model, the proposed experimental implementation is numerically investigated on grounds of the Debye-Wolff integral and dynadic Green function to confirm the predicted chemical interface contrast.<\/jats:p>","DOI":"10.1364\/oe.414972","type":"journal-article","created":{"date-parts":[[2021,1,11]],"date-time":"2021-01-11T02:30:27Z","timestamp":1610332227000},"page":"3985","update-policy":"https:\/\/doi.org\/10.1364\/crossmark_policy","source":"Crossref","is-referenced-by-count":1,"title":["Laser scanning dark-field coherent anti-Stokes Raman scattering (DF-CARS): a numerical study"],"prefix":"10.1364","volume":"29","author":[{"given":"Sandro","family":"Heuke","sequence":"first","affiliation":[{"name":"CNRS"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Herv\u00e9","family":"Rigneault","sequence":"additional","affiliation":[{"name":"CNRS"}],"role":[{"role":"author","vocabulary":"crossref"}]}],"member":"285","published-online":{"date-parts":[[2021,1,25]]},"reference":[{"key":"oe-29-3-3985-R1","first-page":"385","volume":"8","author":"Smith","year":"1955","journal-title":"Research (London)"},{"key":"oe-29-3-3985-R2","first-page":"9","volume":"16","author":"Nomarski","year":"1955","journal-title":"J. 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