{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,9,9]],"date-time":"2026-09-09T20:59:36Z","timestamp":1788987576631,"version":"build-2803163510"},"reference-count":68,"publisher":"Optica Publishing Group","issue":"10","license":[{"start":{"date-parts":[[2024,4,29]],"date-time":"2024-04-29T00:00:00Z","timestamp":1714348800000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/doi.org\/10.1364\/OA_License_v2#VOR-OA"},{"start":{"date-parts":[[2024,4,29]],"date-time":"2024-04-29T00:00:00Z","timestamp":1714348800000},"content-version":"tdm","delay-in-days":0,"URL":"https:\/\/opg.optica.org\/policies\/opg-tdm-policy.json"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["92150101"],"award-info":[{"award-number":["92150101"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100012166","name":"National Key Research and Development Program of China","doi-asserted-by":"publisher","award":["2023YFF0719200"],"award-info":[{"award-number":["2023YFF0719200"]}],"id":[{"id":"10.13039\/501100012166","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100003399","name":"Science and Technology Commission of Shanghai Municipality","doi-asserted-by":"publisher","award":["21JC1402600"],"award-info":[{"award-number":["21JC1402600"]}],"id":[{"id":"10.13039\/501100003399","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":["opg.optica.org"],"crossmark-restriction":false},"short-container-title":["Opt. Express"],"published-print":{"date-parts":[[2024,5,6]]},"abstract":"<jats:p>\n                    Tin diselenide (SnSe\n                    <jats:sub>2<\/jats:sub>\n                    ), a layered transition metal dichalcogenide (TMDC), stands out among other TMDCs for its extraordinary photoactive ability and low thermal conductivity. Consequently, it has stimulated many influential researches on photodetectors, ultrafast pulse shaping, thermoelectric devices, etc. However, the carrier mobility in SnSe\n                    <jats:sub>2<\/jats:sub>\n                    , as determined experimentally, remains limited to tens of cm\n                    <jats:sup>2<\/jats:sup>\n                    V\n                    <jats:sup>-1<\/jats:sup>\n                    s\n                    <jats:sup>-1<\/jats:sup>\n                    . This limitation poses a challenge for achieving high-performance SnSe\n                    <jats:sub>2<\/jats:sub>\n                    -based devices. Theoretical calculations, on the other hand, predict that the carrier mobility in SnSe\n                    <jats:sub>2<\/jats:sub>\n                    can reach hundreds of cm\n                    <jats:sup>2<\/jats:sup>\n                    V\n                    <jats:sup>-1<\/jats:sup>\n                    s\n                    <jats:sup>-1<\/jats:sup>\n                    , approximately one order of magnitude higher than experimental value. Interestingly, the carrier mobility could be underestimated significantly in long-range transportation measurements due to the presence of defects and boundary scattering effects. To address this discrepancy, we employ optic pump terahertz probe spectroscopy to access the photoinduced dynamical THz photoconductivity of SnSe\n                    <jats:sub>2<\/jats:sub>\n                    . Our findings reveal that the intrinsic carrier mobility in conventional SnSe\n                    <jats:sub>2<\/jats:sub>\n                    single crystal is remarkably high, reaching 353.2\u2009\u00b1\u200937.7 cm\n                    <jats:sup>2<\/jats:sup>\n                    V\n                    <jats:sup>-1<\/jats:sup>\n                    s\n                    <jats:sup>-1<\/jats:sup>\n                    , consistent with the theoretical prediction. Additionally, dynamical THz photoconductivity measurements reveal that the SnSe\n                    <jats:sub>2<\/jats:sub>\n                    crystal containing rich defects efficiently capture photoinduced conduction-band electrons and valence-band holes with time constants of \u223c20 and \u223c200 ps, respectively. Meanwhile, we observe an impulsively stimulated Raman scattering at 0.60 THz. Our study not only demonstrates ultrafast THz spectroscopy as a reliable method for determining intrinsic carrier mobility and detection of low frequency coherent Raman mode in materials but also provides valuable reference for the future application of high-performance SnSe\n                    <jats:sub>2<\/jats:sub>\n                    -based devices.\n                  <\/jats:p>","DOI":"10.1364\/oe.523383","type":"journal-article","created":{"date-parts":[[2024,4,19]],"date-time":"2024-04-19T04:00:10Z","timestamp":1713499210000},"page":"17657","update-policy":"https:\/\/doi.org\/10.1364\/crossmark_policy","source":"Crossref","is-referenced-by-count":1,"title":["Highly intrinsic carrier mobility in tin diselenide crystal accessed with ultrafast terahertz spectroscopy"],"prefix":"10.1364","volume":"32","author":[{"given":"Kaiwen","family":"Sun","sequence":"first","affiliation":[{"id":[{"id":"https:\/\/ror.org\/006teas31","id-type":"ROR","asserted-by":"publisher"}]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Wei","family":"Xia","sequence":"additional","affiliation":[{"name":"ShanghaiTech University"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Chen","family":"Wang","sequence":"additional","affiliation":[{"id":[{"id":"https:\/\/ror.org\/006teas31","id-type":"ROR","asserted-by":"publisher"}]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-7692-8014","authenticated-orcid":true,"given":"Peng","family":"Suo","sequence":"additional","affiliation":[{"id":[{"id":"https:\/\/ror.org\/006teas31","id-type":"ROR","asserted-by":"publisher"}]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yuqing","family":"Zou","sequence":"additional","affiliation":[{"id":[{"id":"https:\/\/ror.org\/006teas31","id-type":"ROR","asserted-by":"publisher"}]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jun","family":"Peng","sequence":"additional","affiliation":[{"id":[{"id":"https:\/\/ror.org\/006teas31","id-type":"ROR","asserted-by":"publisher"}]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Wei","family":"Wang","sequence":"additional","affiliation":[{"id":[{"id":"https:\/\/ror.org\/006teas31","id-type":"ROR","asserted-by":"publisher"}]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-1114-4598","authenticated-orcid":true,"given":"Xian","family":"Lin","sequence":"additional","affiliation":[{"id":[{"id":"https:\/\/ror.org\/006teas31","id-type":"ROR","asserted-by":"publisher"}]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9686-7965","authenticated-orcid":true,"given":"Zuanming","family":"Jin","sequence":"additional","affiliation":[{"name":"University of Shanghai for Science and Technology"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yanfeng","family":"Guo","sequence":"additional","affiliation":[{"name":"ShanghaiTech University"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Guohong","family":"Ma","sequence":"additional","affiliation":[{"id":[{"id":"https:\/\/ror.org\/006teas31","id-type":"ROR","asserted-by":"publisher"}]},{"name":"Shanghai University"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"285","published-online":{"date-parts":[[2024,4,29]]},"reference":[{"key":"oe-32-10-17657-R1","doi-asserted-by":"publisher","first-page":"10699","DOI":"10.1038\/srep10699","volume":"5","author":"Iqbal","year":"2015","journal-title":"Sci. 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