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Express"],"published-print":{"date-parts":[[2025,12,15]]},"abstract":"<jats:p>Imparting vivid colors to photovoltaic devices has traditionally required sacrificing power conversion efficiency, a trade-off that limits their adoption in building-integrated photovoltaics (BIPV) and other aesthetics-driven applications. Here, we overcome this constraint by integrating short-range correlated disordered dielectric nanostructures onto high-efficiency organic-silicon heterojunction solar cells. These wavelength-scale nanospheres act dually to suppress broadband specular reflection, thereby enhancing light harvesting, and to generate coherent off-specular scattering that yields iridescent structural colors. To explore this mechanism, we developed a large-scale theoretical framework that decouples collective disorder from single-particle scattering responses, enabling quantitative prediction of the color-efficiency interplay in assemblies of more than 2000 nanoparticles. Experimentally, the iridescent device achieves a power conversion efficiency of 8.17%, compared with 7.3% for the reference device without PS nanospheres, while exhibiting high-saturation CIE 1931 color coordinates. This work demonstrates that vivid coloration does not require strong reflection, overturning the long-standing efficiency-aesthetics trade-off and opening pathways to next-generation BIPV that combine performance with visual appeal.<\/jats:p>","DOI":"10.1364\/oe.580549","type":"journal-article","created":{"date-parts":[[2025,11,19]],"date-time":"2025-11-19T06:00:10Z","timestamp":1763532010000},"page":"52143","update-policy":"https:\/\/doi.org\/10.1364\/crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Breaking the color-efficiency trade-off: aesthetic rainbow organic-silicon solar cell"],"prefix":"10.1364","volume":"33","author":[{"given":"Yi","family":"Yang","sequence":"first","affiliation":[{"id":[{"id":"https:\/\/ror.org\/04ct4d772","id-type":"ROR","asserted-by":"publisher"}]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Dan","family":"Su","sequence":"additional","affiliation":[{"id":[{"id":"https:\/\/ror.org\/04ct4d772","id-type":"ROR","asserted-by":"publisher"}]},{"name":"Southeast University Suzhou Campus"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jun","family":"Wang","sequence":"additional","affiliation":[{"id":[{"id":"https:\/\/ror.org\/04ct4d772","id-type":"ROR","asserted-by":"publisher"}]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Sami","family":"Iqbal","sequence":"additional","affiliation":[{"id":[{"id":"https:\/\/ror.org\/04ct4d772","id-type":"ROR","asserted-by":"publisher"}]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shi-Han","family":"Yang","sequence":"additional","affiliation":[{"id":[{"id":"https:\/\/ror.org\/04ct4d772","id-type":"ROR","asserted-by":"publisher"}]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ze-Xian","family":"Chen","sequence":"additional","affiliation":[{"id":[{"id":"https:\/\/ror.org\/04ct4d772","id-type":"ROR","asserted-by":"publisher"}]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Pan-Qin","family":"Sun","sequence":"additional","affiliation":[{"id":[{"id":"https:\/\/ror.org\/04ct4d772","id-type":"ROR","asserted-by":"publisher"}]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shan-Jiang","family":"Wang","sequence":"additional","affiliation":[{"id":[{"id":"https:\/\/ror.org\/04ct4d772","id-type":"ROR","asserted-by":"publisher"}]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yuan-Jun","family":"Song","sequence":"additional","affiliation":[{"id":[{"id":"https:\/\/ror.org\/04ct4d772","id-type":"ROR","asserted-by":"publisher"}]}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-1462-6402","authenticated-orcid":true,"given":"Weiping","family":"Wu","sequence":"additional","affiliation":[{"name":"Chinese Academy of Sciences"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Tong","family":"Zhang","sequence":"additional","affiliation":[{"id":[{"id":"https:\/\/ror.org\/04ct4d772","id-type":"ROR","asserted-by":"publisher"}]},{"name":"Southeast University Suzhou Campus"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"285","published-online":{"date-parts":[[2025,12,2]]},"reference":[{"key":"oe-33-25-52143-R1","doi-asserted-by":"publisher","first-page":"2000613","DOI":"10.1002\/adma.202000631","type":"journal-article","volume":"32","author":"Batmunkh","year":"2020","journal-title":"Adv. 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