{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,13]],"date-time":"2026-10-13T01:57:26Z","timestamp":1791856646659,"version":"4.3.4"},"reference-count":73,"publisher":"Public Library of Science (PLoS)","issue":"2","license":[{"start":{"date-parts":[[2025,2,11]],"date-time":"2025-02-11T00:00:00Z","timestamp":1739232000000},"content-version":"vor","delay-in-days":0,"URL":"http:\/\/creativecommons.org\/licenses\/by\/4.0\/"}],"content-domain":{"domain":["www.plosone.org"],"crossmark-restriction":false},"short-container-title":["PLoS ONE"],"abstract":"<jats:p>This study investigates the fabrication of large-area, highly-ordered monolayers of PbTe quantum dots (QDs) on TiO<jats:sub>2<\/jats:sub>\/ITO substrate, using a fast, simple, and repeatable spin-coating technique. For the first time, a real monolayer (a layer with the height of a single QD) covering approximately 3 cm<jats:sup>2<\/jats:sup> was successfully prepared, achieving a root-mean-square roughness (Rq) of 1.37 nm. The research systematically explores key parameters such as QD morphology, concentration, spin-coating conditions, substrate characteristics, wetting properties, and solvent effects to optimize thin film deposition. The findings reveal that the spin-coating method favors the formation of layers with spherical QDs (6\u20139 nm) over cubical QDs (10\u201313 nm). The findings highlight the significant influence of solvent evaporation rate, viscosity, and wettability on monolayer quality. Chloroform was identified as the optimal solvent for cubical QDs (~90% coverage), while hexane was more effective for spherical QDs (90%-100% coverage). Beyond monolayers, high-quality bilayers were also fabricated, demonstrating the method\u2019s potential for multilayer fabrication. This rapid and efficient method for monolayer and bilayer fabrication marks a significant breakthrough in producing uniform, large-area films, facilitating seamless integration with existing technologies. It offers a scalable and cost-effective solution, opening the door to broader applications in fields that demand high-quality thin film deposition.<\/jats:p>","DOI":"10.1371\/journal.pone.0317677","type":"journal-article","created":{"date-parts":[[2025,2,11]],"date-time":"2025-02-11T18:28:01Z","timestamp":1739298481000},"page":"e0317677","update-policy":"https:\/\/doi.org\/10.1371\/journal.pone.corrections_policy","source":"Crossref","is-referenced-by-count":4,"title":["PbTe quantum dots highly packed monolayer fabrication by a spin coating method"],"prefix":"10.1371","volume":"20","author":[{"ORCID":"https:\/\/orcid.org\/0000-0001-8778-0246","authenticated-orcid":true,"given":"Svetlana","family":"Lyssenko","sequence":"first","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Michal","family":"Amar","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-3907-5267","authenticated-orcid":true,"given":"Alina","family":"Sermiagin","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-1857-4905","authenticated-orcid":true,"given":"Refael","family":"Minnes","sequence":"additional","affiliation":[],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"340","published-online":{"date-parts":[[2025,2,11]]},"reference":[{"key":"pone.0317677.ref001","doi-asserted-by":"crossref","first-page":"121828","DOI":"10.1016\/j.talanta.2020.121828","article-title":"A critical review on quantum dots: From synthesis toward applications in electrochemical biosensors for determination of disease-related biomolecules","volume":"224","author":"MA Farzin","year":"2021","journal-title":"Talanta"},{"key":"pone.0317677.ref002","doi-asserted-by":"crossref","first-page":"141399","DOI":"10.1016\/j.cej.2023.141399","article-title":"Recent advances in quantum dots photocatalysts","volume":"458","author":"P Sun","year":"2023","journal-title":"Chemical Engineering Journal"},{"key":"pone.0317677.ref003","doi-asserted-by":"crossref","first-page":"6882","DOI":"10.1021\/acsanm.8b01696","article-title":"Comparing Halide Ligands in PbS Colloidal Quantum Dots for Field-Effect Transistors and Solar Cells","volume":"1","author":"D Bederak","year":"2018","journal-title":"ACS Appl Nano Mater"},{"key":"pone.0317677.ref004","doi-asserted-by":"crossref","first-page":"1139","DOI":"10.3390\/cryst13071139","article-title":"Next-Generation Quantum Materials for Thermoelectric Energy Conversion","volume":"13","author":"SK Singh","year":"2023","journal-title":"Crystals (Basel)"},{"key":"pone.0317677.ref005","doi-asserted-by":"crossref","first-page":"2107532","DOI":"10.1002\/adma.202107532","article-title":"Low-Threshold, Highly Stable Colloidal Quantum Dot Short-Wave Infrared Laser enabled by Suppression of Trap-Assisted Auger Recombination","volume":"34","author":"N Taghipour","year":"2022","journal-title":"Advanced Materials"},{"key":"pone.0317677.ref006","first-page":"1","article-title":"Semiconducting Quantum Dots for Energy Conversion and Storage","volume":"2213770","author":"Y Yu","year":"2023","journal-title":"Adv Funct Mater"},{"key":"pone.0317677.ref007","doi-asserted-by":"crossref","first-page":"1908762","DOI":"10.1002\/adfm.201908762","article-title":"Core\/Shell Quantum Dots Solar Cells","volume":"30","author":"GS Selopal","year":"2020","journal-title":"Adv Funct Mater"},{"key":"pone.0317677.ref008","doi-asserted-by":"crossref","first-page":"2433","DOI":"10.1080\/25740881.2024.2375363","article-title":"Graphene Quantum Dots Nanocomposite Membranes\u2014State-of-the-art and Next-Generation Potential","volume":"63","author":"A. 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