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Tricalcium silicate (C3S), the primary phase in Portland cement, is known to have complex dissolution mechanisms that involve multiple reactions and changes to particle surfaces. As a result, current analytical models are unable to accurately predict the dissolution kinetics of C3S in various solvents when it is undersaturated with respect to the solvent. This paper employs the deep forest (DF) model to predict the dissolution rate of C3S in the undersaturated solvent. The DF model takes into account several variables, including the measurement method (i.e., reactor connected to inductive coupled plasma spectrometer and flow chamber with vertical scanning interferometry), temperature, and physicochemical properties of solvents. Next, the DF model evaluates the influence of each variable on the dissolution rate of C3S, and this information is used to develop a closed-form analytical model that can predict the dissolution rate of C3S. The coefficients and constant of the analytical model are optimized in two scenarios: generic and alkaline solvents. The results show that both the DF and analytical models are able to produce reliable predictions of the dissolution rate of C3S when it is undersaturated and far from equilibrium.<\/jats:p>","DOI":"10.3390\/a16010007","type":"journal-article","created":{"date-parts":[[2022,12,22]],"date-time":"2022-12-22T03:24:30Z","timestamp":1671679470000},"page":"7","update-policy":"https:\/\/doi.org\/10.3390\/mdpi_crossmark_policy","source":"Crossref","is-referenced-by-count":4,"title":["Predicting Dissolution Kinetics of Tricalcium Silicate Using Deep Learning and Analytical Models"],"prefix":"10.3390","volume":"16","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-7111-5206","authenticated-orcid":false,"given":"Taihao","family":"Han","sequence":"first","affiliation":[{"name":"Department of Materials Science and Engineering, Missouri University of Science and Technology, Rolla, MO 65409, USA"}]},{"given":"Sai Akshay","family":"Ponduru","sequence":"additional","affiliation":[{"name":"Department of Materials Science and Engineering, Missouri University of Science and Technology, Rolla, MO 65409, USA"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-6419-2270","authenticated-orcid":false,"given":"Arianit","family":"Reka","sequence":"additional","affiliation":[{"name":"Department of Materials Science and Engineering, Missouri University of Science and Technology, Rolla, MO 65409, USA"},{"name":"Faculty of Natural Sciences and Mathematics, University of Tetova, 1220 Tetovo, North Macedonia"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-8659-2910","authenticated-orcid":false,"given":"Jie","family":"Huang","sequence":"additional","affiliation":[{"name":"Department of Electrical and Computer Engineering, Missouri University of Science and Technology, Rolla, MO 65409, USA"}]},{"given":"Gaurav","family":"Sant","sequence":"additional","affiliation":[{"name":"Civil and Environmental Engineering, University of California, Los Angeles, CA 90095, USA"}]},{"given":"Aditya","family":"Kumar","sequence":"additional","affiliation":[{"name":"Department of Materials Science and Engineering, Missouri University of Science and Technology, Rolla, MO 65409, USA"}]}],"member":"1968","published-online":{"date-parts":[[2022,12,22]]},"reference":[{"key":"ref_1","doi-asserted-by":"crossref","first-page":"126","DOI":"10.1016\/j.cemconres.2015.04.012","article-title":"A Review of Alternative Approaches to the Reduction of CO2 Emissions Associated with the Manufacture of the Binder Phase in Concrete","volume":"78","author":"Gartner","year":"2015","journal-title":"Cem. 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