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By systematic optimal control study, via the Pontryagin maximum principle, we design alternative more efficient routes that, for a given admissible loss, feature an optimal transfer with respect to the cost defined as (i) the pulse energy (energy minimization) or (ii) the pulse duration (time minimization). The optimal controls feature remarkably simple sequences in the respective cases: (i) operating far from a dark state, of \u03c0-pulse type in the limit of low admissible loss, or (ii) close to the dark state with a counterintuitive pulse configuration sandwiched by sharp intuitive sequences, referred to as the intuitive\/counterintuitive\/intuitive (ICI) sequence. In the case of time optimization, the resulting stimulated Raman exact passage (STIREP) outperforms STIRAP in term of speed, accuracy, and robustness for low admissible loss.<\/jats:p>","DOI":"10.3390\/e25050790","type":"journal-article","created":{"date-parts":[[2023,5,12]],"date-time":"2023-05-12T09:56:18Z","timestamp":1683885378000},"page":"790","update-policy":"https:\/\/doi.org\/10.3390\/mdpi_crossmark_policy","source":"Crossref","is-referenced-by-count":9,"title":["Optimal Pulse Design for Dissipative-Stimulated Raman Exact Passage"],"prefix":"10.3390","volume":"25","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-5642-8458","authenticated-orcid":false,"given":"Kaipeng","family":"Liu","sequence":"first","affiliation":[{"name":"Laboratoire Interdisciplinaire Carnot de Bourgogne, CNRS UMR 6303, Universit\u00e9 de Bourgogne, BP 47870, 21078 Dijon, France"},{"name":"International Center of Quantum Artificial Intelligence for Science and Technology (QuArtist), Department of Physics, Shanghai University, Shanghai 200444, China"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-1963-333X","authenticated-orcid":false,"given":"Dominique","family":"Sugny","sequence":"additional","affiliation":[{"name":"Laboratoire Interdisciplinaire Carnot de Bourgogne, CNRS UMR 6303, Universit\u00e9 de Bourgogne, BP 47870, 21078 Dijon, France"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-4221-4288","authenticated-orcid":false,"given":"Xi","family":"Chen","sequence":"additional","affiliation":[{"name":"Department of Physical Chemistry, University of the Basque Country UPV\/EHU, Apartado 644, 48080 Bilbao, Spain"},{"name":"EHU Quantum Center, University of the Basque Country UPV\/EHU, Barrio Sarriena, s\/n, 48940 Leioa, Spain"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9826-9598","authenticated-orcid":false,"given":"St\u00e9phane","family":"Gu\u00e9rin","sequence":"additional","affiliation":[{"name":"Laboratoire Interdisciplinaire Carnot de Bourgogne, CNRS UMR 6303, Universit\u00e9 de Bourgogne, BP 47870, 21078 Dijon, France"}]}],"member":"1968","published-online":{"date-parts":[[2023,5,12]]},"reference":[{"key":"ref_1","unstructured":"Nielsen, M.A., and Chuang, I.L. 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