{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,6,27]],"date-time":"2026-06-27T19:56:16Z","timestamp":1782590176209,"version":"3.54.5"},"reference-count":46,"publisher":"MDPI AG","issue":"8","license":[{"start":{"date-parts":[[2020,4,18]],"date-time":"2020-04-18T00:00:00Z","timestamp":1587168000000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/creativecommons.org\/licenses\/by\/4.0\/"}],"funder":[{"name":"Department of Energy National Nuclear Security Administration, Department of Energy National Nuclear Security Administration, Consortium for Monitoring, Verification, and Technology","award":["DE-NE000863"],"award-info":[{"award-number":["DE-NE000863"]}]},{"name":"Department of Energy National Nuclear Security Administration, Consortium for Verification Technology","award":["DE-NA0002534"],"award-info":[{"award-number":["DE-NA0002534"]}]},{"DOI":"10.13039\/100000181","name":"Air Force Office of Scientific Research","doi-asserted-by":"publisher","award":["FA9550-16-1-0121"],"award-info":[{"award-number":["FA9550-16-1-0121"]}],"id":[{"id":"10.13039\/100000181","id-type":"DOI","asserted-by":"publisher"}]},{"name":"National Science Foundation Graduate Research Fellowship Program","award":["DGE 1256260"],"award-info":[{"award-number":["DGE 1256260"]}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":["Remote Sensing"],"abstract":"<jats:p>Optical measurement techniques can address certain important challenges associated with nuclear safety and security. Detection of uranium over long distances presents one such challenge that is difficult to realize with traditional ionizing radiation detection, but may benefit from the use of techniques based on intense femtosecond laser pulses. When a high-power laser pulse propagates in air, it experiences collapse and confinement into filaments over an extended distance even without external focusing. In our experiments, we varied the initial pulse chirp to optimize the emission signal from the laser-produced uranium plasma at an extended distance. While the ablation efficiency of filaments formed by self-focusing is known to be significantly lower when compared to filaments produced by external focusing, we show that filaments formed by self-focusing can still generate luminous spectroscopic signatures of uranium detectable within seconds over a 10-m range. The intensity of uranium emission varies periodically with laser chirp, which is attributed to the interplay among self-focusing, defocusing, and multi-filament fragmentation along the beam propagation axis. Grouping of multi-filaments incident on target is found to be correlated with the uranium emission intensity. The results show promise towards long-range detection, advancing the diagnostics and analytical capabilities in ultrafast laser-based spectroscopy of high-Z elements.<\/jats:p>","DOI":"10.3390\/rs12081281","type":"journal-article","created":{"date-parts":[[2020,4,21]],"date-time":"2020-04-21T04:49:38Z","timestamp":1587444578000},"page":"1281","update-policy":"https:\/\/doi.org\/10.3390\/mdpi_crossmark_policy","source":"Crossref","is-referenced-by-count":18,"title":["Remote Detection of Uranium Using Self-Focusing Intense Femtosecond Laser Pulses"],"prefix":"10.3390","volume":"12","author":[{"given":"Milo\u0161","family":"Burger","sequence":"first","affiliation":[{"name":"Department of Nuclear Engineering and Radiological Sciences, University of Michigan, Ann Arbor, MI 48109, USA"},{"name":"G\u00e9rard Mourou Center for Ultrafast Optical Science, University of Michigan, Ann Arbor, MI 48109, USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-3324-9641","authenticated-orcid":false,"given":"Patrick J.","family":"Skrodzki","sequence":"additional","affiliation":[{"name":"Department of Nuclear Engineering and Radiological Sciences, University of Michigan, Ann Arbor, MI 48109, USA"},{"name":"G\u00e9rard Mourou Center for Ultrafast Optical Science, University of Michigan, Ann Arbor, MI 48109, USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-1811-4968","authenticated-orcid":false,"given":"Lauren A.","family":"Finney","sequence":"additional","affiliation":[{"name":"Department of Nuclear Engineering and Radiological Sciences, University of Michigan, Ann Arbor, MI 48109, USA"},{"name":"G\u00e9rard Mourou Center for Ultrafast Optical Science, University of Michigan, Ann Arbor, MI 48109, USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"John","family":"Nees","sequence":"additional","affiliation":[{"name":"G\u00e9rard Mourou Center for Ultrafast Optical Science, University of Michigan, Ann Arbor, MI 48109, USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-0573-3150","authenticated-orcid":false,"given":"Igor","family":"Jovanovic","sequence":"additional","affiliation":[{"name":"Department of Nuclear Engineering and Radiological Sciences, University of Michigan, Ann Arbor, MI 48109, USA"},{"name":"G\u00e9rard Mourou Center for Ultrafast Optical Science, University of Michigan, Ann Arbor, MI 48109, USA"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"1968","published-online":{"date-parts":[[2020,4,18]]},"reference":[{"key":"ref_1","doi-asserted-by":"crossref","first-page":"2988","DOI":"10.1038\/srep02988","article-title":"Plutonium release from Fukushima Daiichi fosters the need for more detailed investigations","volume":"3","author":"Schneider","year":"2013","journal-title":"Sci. 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