{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,8,18]],"date-time":"2026-08-18T04:33:31Z","timestamp":1787027611175,"version":"build-2736575974"},"reference-count":70,"publisher":"MDPI AG","issue":"8","license":[{"start":{"date-parts":[[2020,8,11]],"date-time":"2020-08-11T00:00:00Z","timestamp":1597104000000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/creativecommons.org\/licenses\/by\/4.0\/"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["21677038"],"award-info":[{"award-number":["21677038"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"name":"National Basic Research Program of China (973 Program)","award":["2016YFA060130X"],"award-info":[{"award-number":["2016YFA060130X"]}]},{"name":"Major Program of Shanghai Committee of Science and Technology, China","award":["19DZ1205009"],"award-info":[{"award-number":["19DZ1205009"]}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":["Atmosphere"],"abstract":"<jats:p>Marine biogenic dimethyl sulfide (DMS) is an important natural source of sulfur in the atmosphere, which may play an important role in air quality. In this study, the WRF-CMAQ model is employed to assess the impact of DMS on the atmospheric environment at the regional scale of eastern coastal China and urban scale of Shanghai in 2017. A national scale database of DMS concentration in seawater is established based on the historical DMS measurements in the Yellow Sea, the Bohai Sea and the East China Sea in different seasons during 2009~2017. Results indicate that the sea-to-air emission flux of DMS varies greatly in different seasons, with the highest in summer, followed by spring and autumn, and the lowest in winter. The annual DMS emissions from the Yellow Sea, the Bohai Sea and the East China Sea are 0.008, 0.059, and 0.15 Tg S a\u22121, respectively. At the regional scale, DMS emissions increase atmospheric sulfur dioxide (SO2) and sulfate (SO42\u2212) concentrations over the East China seas by a maximum of 8% in summer and a minimum of 2% in winter, respectively. At the urban scale, the addition of DMS emissions increase the SO2 and SO42\u2212 levels by 2% and 5%, respectively, and reduce ozone (O3) in the air of Shanghai by 1.5%~2.5%. DMS emissions increase fine-mode ammonium particle concentration distribution by 4% and 5%, and fine-mode nss-SO42\u2212 concentration distributions by 4% and 9% in the urban and marine air, respectively. Our results indicate that although anthropogenic sources are still the dominant contributor of atmospheric sulfur burden in China, biogenic DMS emissions source cannot be ignored.<\/jats:p>","DOI":"10.3390\/atmos11080849","type":"journal-article","created":{"date-parts":[[2020,8,11]],"date-time":"2020-08-11T09:28:57Z","timestamp":1597138137000},"page":"849","update-policy":"https:\/\/doi.org\/10.3390\/mdpi_crossmark_policy","source":"Crossref","is-referenced-by-count":18,"title":["Regional and Urban-Scale Environmental Influences of Oceanic DMS Emissions over Coastal China Seas"],"prefix":"10.3390","volume":"11","author":[{"given":"Shanshan","family":"Li","sequence":"first","affiliation":[{"name":"Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP3), Department of Environmental Science and Engineering, Fudan University, Shanghai 200438, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yan","family":"Zhang","sequence":"additional","affiliation":[{"name":"Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP3), Department of Environmental Science and Engineering, Fudan University, Shanghai 200438, China"},{"name":"Big Data Institute for Carbon Emission and Environmental Pollution, Fudan University, Shanghai 200433, China"},{"name":"Institute of Atmospheric Sciences, Fudan University, Shanghai 200438, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-5464-8660","authenticated-orcid":false,"given":"Junri","family":"Zhao","sequence":"additional","affiliation":[{"name":"Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP3), Department of Environmental Science and Engineering, Fudan University, Shanghai 200438, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Golam","family":"Sarwar","sequence":"additional","affiliation":[{"name":"Center for Environmental Measurement and Modeling, Office of Research and Development, U.S. Environmental Protection Agency, Research Triangle Park, NC 27711, USA"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-0846-0127","authenticated-orcid":false,"given":"Shengqian","family":"Zhou","sequence":"additional","affiliation":[{"name":"Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP3), Department of Environmental Science and Engineering, Fudan University, Shanghai 200438, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ying","family":"Chen","sequence":"additional","affiliation":[{"name":"Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP3), Department of Environmental Science and Engineering, Fudan University, Shanghai 200438, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Guipeng","family":"Yang","sequence":"additional","affiliation":[{"name":"Key Laboratory of Marine Chemistry Theory and Technology, Ministry of Education, College of Chemistry and Chemical Engineering, Ocean University of China, Qingdao 266100, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-0060-1581","authenticated-orcid":false,"given":"Alfonso","family":"Saiz-Lopez","sequence":"additional","affiliation":[{"name":"Department of Atmospheric Chemistry and Climate, Institute of Physical Chemistry Rocasolano, CSIC, 28006 Madrid, Spain"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"1968","published-online":{"date-parts":[[2020,8,11]]},"reference":[{"key":"ref_1","doi-asserted-by":"crossref","first-page":"744","DOI":"10.1126\/science.221.4612.744","article-title":"Dimethyl sulfide in the surface ocean and the marine atmosphere\u2014A global view","volume":"221","author":"Andreae","year":"1983","journal-title":"Science"},{"key":"ref_2","doi-asserted-by":"crossref","first-page":"315","DOI":"10.1007\/BF00115242","article-title":"Sulfur emissions to the atmosphere from natural sources","volume":"14","author":"Bates","year":"1992","journal-title":"J. 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