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The synergistic effect of various metal compounds immobilized on conductive substrates has been considered for wastewater treatment. However, developing a facile and universal approach for rational design and enhancing photocatalytic properties has endured extreme challenges. Herein, we develop a strategy to facilitate the photocatalytic reactions by designing a composite architecture of ZIF\u20138 ligand binding to the in\u2013situ synthesis ZnO seed layer on carbon fiber. In this architecture, the dissolution and release of the seed layer in the excessive 2\u2013Methylimidazole methanol solution were used as the binder to enhance the interplay between organic ligand and substrate. As an evaluated system for antibiotic contaminants, the photodegradation of tetracycline hydrochloride was performed with a removal efficiency of 88.47% (TC = 50 mg\/L, pH = 4, 0.08 g of photocatalyst, illumination within 100 min). Moreover, the photocatalyst exhibited a steady photocatalytic activity (75.0%) after five cycles. The present work demonstrated a strategy for enhancing the photocatalytic performances of carbon fiber and accordingly provided useful perception into the design of the synergistic structure.<\/jats:p>","DOI":"10.3390\/ijms231911286","type":"journal-article","created":{"date-parts":[[2022,9,25]],"date-time":"2022-09-25T23:13:27Z","timestamp":1664147607000},"page":"11286","update-policy":"https:\/\/doi.org\/10.3390\/mdpi_crossmark_policy","source":"Crossref","is-referenced-by-count":4,"title":["Metal\u2013Organic Frameworks Meet Metallic Oxide on Carbon Fiber: Synergistic Effect for Enhanced Photodegradation of Antibiotic Pollutant"],"prefix":"10.3390","volume":"23","author":[{"given":"Na","family":"Zhu","sequence":"first","affiliation":[{"name":"State Key Laboratory of New Textile Materials and Advanced Processing Technologies, Wuhan Textile University, Wuhan 430200, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Sijie","family":"Zhou","sequence":"additional","affiliation":[{"name":"State Key Laboratory of New Textile Materials and Advanced Processing Technologies, Wuhan Textile University, Wuhan 430200, China"},{"name":"College of Textiles, Donghua University, Shanghai 201620, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Chunhua","family":"Zhang","sequence":"additional","affiliation":[{"name":"State Key Laboratory of New Textile Materials and Advanced Processing Technologies, Wuhan Textile University, Wuhan 430200, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Zhuan","family":"Fu","sequence":"additional","affiliation":[{"name":"State Key Laboratory of New Textile Materials and Advanced Processing Technologies, Wuhan Textile University, Wuhan 430200, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Junyao","family":"Gong","sequence":"additional","affiliation":[{"name":"State Key Laboratory of New Textile Materials and Advanced Processing Technologies, Wuhan Textile University, Wuhan 430200, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Zhaozixuan","family":"Zhou","sequence":"additional","affiliation":[{"name":"State Key Laboratory of New Textile Materials and Advanced Processing Technologies, Wuhan Textile University, Wuhan 430200, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Xiaofeng","family":"Wang","sequence":"additional","affiliation":[{"name":"State Key Laboratory of New Textile Materials and Advanced Processing Technologies, Wuhan Textile University, Wuhan 430200, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Pei","family":"Lyu","sequence":"additional","affiliation":[{"name":"Institute for Frontier Materials, Deakin University, Geelong, VIC 3216, Australia"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-0622-4497","authenticated-orcid":false,"given":"Li","family":"Li","sequence":"additional","affiliation":[{"name":"Institute of Textiles and Clothing, The Hong Kong Polytechnic University, Hong Kong 999077, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-1514-6702","authenticated-orcid":false,"given":"Liangjun","family":"Xia","sequence":"additional","affiliation":[{"name":"State Key Laboratory of New Textile Materials and Advanced Processing Technologies, Wuhan Textile University, Wuhan 430200, China"},{"name":"Institute of Textiles and Clothing, The Hong Kong Polytechnic University, Hong Kong 999077, China"}],"role":[{"role":"author","vocabulary":"crossref"}]}],"member":"1968","published-online":{"date-parts":[[2022,9,25]]},"reference":[{"key":"ref_1","doi-asserted-by":"crossref","first-page":"132114","DOI":"10.1016\/j.cej.2021.132114","article-title":"Circular economy is game\u2013changing municipal wastewater treatment technology towards energy and carbon neutrality","volume":"429","author":"Zhang","year":"2022","journal-title":"Chem. 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