{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,1,17]],"date-time":"2026-01-17T15:58:28Z","timestamp":1768665508434,"version":"3.49.0"},"reference-count":59,"publisher":"MDPI AG","issue":"2","license":[{"start":{"date-parts":[[2026,1,14]],"date-time":"2026-01-14T00:00:00Z","timestamp":1768348800000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/creativecommons.org\/licenses\/by\/4.0\/"}],"funder":[{"DOI":"10.13039\/501100001809","name":"the National Natural Science Foundation of China","doi-asserted-by":"crossref","award":["52231007"],"award-info":[{"award-number":["52231007"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"crossref"}]},{"DOI":"10.13039\/501100001809","name":"the National Natural Science Foundation of China","doi-asserted-by":"crossref","award":["12327804"],"award-info":[{"award-number":["12327804"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"crossref"}]},{"DOI":"10.13039\/501100001809","name":"the National Natural Science Foundation of China","doi-asserted-by":"crossref","award":["T2321003"],"award-info":[{"award-number":["T2321003"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"crossref"}]},{"DOI":"10.13039\/501100001809","name":"the National Natural Science Foundation of China","doi-asserted-by":"crossref","award":["22088101"],"award-info":[{"award-number":["22088101"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"crossref"}]},{"DOI":"10.13039\/501100001809","name":"the National Natural Science Foundation of China","doi-asserted-by":"crossref","award":["22405050"],"award-info":[{"award-number":["22405050"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"crossref"}]},{"name":"the National Key Research Program of China","award":["2024YFA1208902"],"award-info":[{"award-number":["2024YFA1208902"]}]},{"name":"the National Key Research Program of China","award":["2024YFA1408000"],"award-info":[{"award-number":["2024YFA1408000"]}]},{"name":"the National Key Research Program of China","award":["2021YFA1200600"],"award-info":[{"award-number":["2021YFA1200600"]}]},{"name":"the Science and Technology Commission of Shanghai Municipality","award":["24ZR1406400"],"award-info":[{"award-number":["24ZR1406400"]}]},{"name":"Key Laboratory of High Temperature Electromagnetic Materials and Structure of MOE","award":["KB202401"],"award-info":[{"award-number":["KB202401"]}]},{"name":"Fund of Science and Technology on Surface Physics and Chemistry Laboratory","award":["JCKYS2023120201"],"award-info":[{"award-number":["JCKYS2023120201"]}]},{"DOI":"10.13039\/501100003395","name":"Shanghai Municipal Education Commission","doi-asserted-by":"publisher","award":["24KXZNA06"],"award-info":[{"award-number":["24KXZNA06"]}],"id":[{"id":"10.13039\/501100003395","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":["Materials"],"abstract":"<jats:p>Two-dimensional ferromagnets are promising for compact spintronic devices. However, their centrosymmetric structure inherently suppresses the Dzyaloshinskii\u2013Moriya interaction (DMI), hindering the stabilization of chiral spin texture. Here, a tunable DMI induced by interface symmetry breaking in Fe3GeTe2\/MoS2 vdW heterostructures is reported. We find that the interfacial DMI stabilizes N\u00e9el-type skyrmions in Fe3GeTe2\/MoS2 heterostructures under zero magnetic field, with nucleation observed at 64 Oe and annihilation at 800 Oe via Lorentz transmission electron microscopy (LTEM). Skyrmion density peaks (~0.57 skyrmions\/\u03bcm2) at a Fe3GeTe2 thickness of ~30 nm and decays beyond ~60 nm, indicating a finite penetration depth of the proximity effect. Such modulated DMI enables a stabilized nucleation of N\u00e9el type skyrmions, allowing for precise control over their density, revealed by Lorentz transmission electron microscopy. Thickness-dependent measurements confirm the interfacial origin of this stabilization. Skyrmion density reaches peak in thin Fe3GeTe2 layers and decays beyond ~60 nm, defining the finite penetration depth of the proximity effect. Micromagnetic simulations reproduce the field-dependent evolution of skyrmions, showing a strong correlation to interfacial DMI. First-principles calculations attribute this DMI to asymmetric charge redistribution and spin\u2013orbit coupling at the heterointerface. This work establishes interface engineering as a universal strategy for stabilizing skyrmions in centrosymmetric vdW ferromagnets, offering a thickness-tunable platform for next-generation two-dimensional spintronic devices.<\/jats:p>","DOI":"10.3390\/ma19020340","type":"journal-article","created":{"date-parts":[[2026,1,15]],"date-time":"2026-01-15T08:26:36Z","timestamp":1768465596000},"page":"340","update-policy":"https:\/\/doi.org\/10.3390\/mdpi_crossmark_policy","source":"Crossref","is-referenced-by-count":0,"title":["Creation of High-Density N\u00e9el Skyrmions by Interfacial-Proximity Engineering"],"prefix":"10.3390","volume":"19","author":[{"given":"Tingjia","family":"Zhang","sequence":"first","affiliation":[{"name":"School of Materials and Chemistry, University of Shanghai for Science and Technology, Shanghai 200093, China"},{"name":"Laboratory of Advanced Materials, Shanghai Key Lab of Molecular Catalysis and Innovative Materials, State Key Laboratory of Coatings for Advanced Equipment, College of Smart Materials and Future Energy, Fudan University, Shanghai 200438, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Chendi","family":"Yang","sequence":"additional","affiliation":[{"name":"Laboratory of Advanced Materials, Shanghai Key Lab of Molecular Catalysis and Innovative Materials, State Key Laboratory of Coatings for Advanced Equipment, College of Smart Materials and Future Energy, Fudan University, Shanghai 200438, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Xiaowei","family":"Lv","sequence":"additional","affiliation":[{"name":"Laboratory of Advanced Materials, Shanghai Key Lab of Molecular Catalysis and Innovative Materials, State Key Laboratory of Coatings for Advanced Equipment, College of Smart Materials and Future Energy, Fudan University, Shanghai 200438, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Ke","family":"Pei","sequence":"additional","affiliation":[{"name":"Electron Microscopy Center, Institute of Science and Technology, Fudan University, Shanghai 200438, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Xiao","family":"Yang","sequence":"additional","affiliation":[{"name":"Laboratory of Advanced Materials, Shanghai Key Lab of Molecular Catalysis and Innovative Materials, State Key Laboratory of Coatings for Advanced Equipment, College of Smart Materials and Future Energy, Fudan University, Shanghai 200438, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Wuyang","family":"Tan","sequence":"additional","affiliation":[{"name":"Laboratory of Advanced Materials, Shanghai Key Lab of Molecular Catalysis and Innovative Materials, State Key Laboratory of Coatings for Advanced Equipment, College of Smart Materials and Future Energy, Fudan University, Shanghai 200438, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Junye","family":"Pan","sequence":"additional","affiliation":[{"name":"College of Physics, Donghua University, Shanghai 201620, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Jiazhuan","family":"Qin","sequence":"additional","affiliation":[{"name":"Laboratory of Advanced Materials, Shanghai Key Lab of Molecular Catalysis and Innovative Materials, State Key Laboratory of Coatings for Advanced Equipment, College of Smart Materials and Future Energy, Fudan University, Shanghai 200438, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0009-0009-9395-1801","authenticated-orcid":false,"given":"Meichen","family":"Wen","sequence":"additional","affiliation":[{"name":"Materials Genome Institute, Shanghai University, Shanghai 200444, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-8224-0590","authenticated-orcid":false,"given":"Wei","family":"Li","sequence":"additional","affiliation":[{"name":"School of Materials and Chemistry, University of Shanghai for Science and Technology, Shanghai 200093, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-4352-1581","authenticated-orcid":false,"given":"Jia","family":"Liang","sequence":"additional","affiliation":[{"name":"College of Smart Materials and Future Energy, State Key Laboratory of Photovoltaic Science and Technology, Fudan University, Shanghai 200433, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-6583-7114","authenticated-orcid":false,"given":"Renchao","family":"Che","sequence":"additional","affiliation":[{"name":"Laboratory of Advanced Materials, Shanghai Key Lab of Molecular Catalysis and Innovative Materials, State Key Laboratory of Coatings for Advanced Equipment, College of Smart Materials and Future Energy, Fudan University, Shanghai 200438, China"}],"role":[{"role":"author","vocabulary":"crossref"}]}],"member":"1968","published-online":{"date-parts":[[2026,1,14]]},"reference":[{"key":"ref_1","doi-asserted-by":"crossref","first-page":"554","DOI":"10.1038\/s41565-018-0186-z","article-title":"Electric-field control of magnetism in a few-layered van der Waals ferromagnetic semiconductor","volume":"13","author":"Wang","year":"2018","journal-title":"Nat. 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