{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,10,3]],"date-time":"2026-10-03T08:33:48Z","timestamp":1791016428102,"version":"4.1.0"},"reference-count":54,"publisher":"MDPI AG","issue":"1","license":[{"start":{"date-parts":[[2023,1,2]],"date-time":"2023-01-02T00:00:00Z","timestamp":1672617600000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/creativecommons.org\/licenses\/by\/4.0\/"}],"funder":[{"name":"National Natural Science Foundation of China","award":["32071702"],"award-info":[{"award-number":["32071702"]}]},{"name":"National Natural Science Foundation of China","award":["31901255"],"award-info":[{"award-number":["31901255"]}]},{"name":"National Natural Science Foundation of China","award":["2019JQ03004"],"award-info":[{"award-number":["2019JQ03004"]}]},{"DOI":"10.13039\/501100012138","name":"Beijing Forestry University Outstanding Young Talent Cultivation Project","doi-asserted-by":"publisher","award":["32071702"],"award-info":[{"award-number":["32071702"]}],"id":[{"id":"10.13039\/501100012138","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100012138","name":"Beijing Forestry University Outstanding Young Talent Cultivation Project","doi-asserted-by":"publisher","award":["31901255"],"award-info":[{"award-number":["31901255"]}],"id":[{"id":"10.13039\/501100012138","id-type":"DOI","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100012138","name":"Beijing Forestry University Outstanding Young Talent Cultivation Project","doi-asserted-by":"publisher","award":["2019JQ03004"],"award-info":[{"award-number":["2019JQ03004"]}],"id":[{"id":"10.13039\/501100012138","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":["Nanomaterials"],"abstract":"<jats:p>Eco-friendly soybean protein adhesives could be an ideal substitute for replacing traditional formaldehyde-based adhesives in wood industry. However, a large number of cross-linking agents are required in soy protein adhesive formulations to obtain sufficiently performing properties. Inspired by the high performance of nacre and branched structures, a hyper-branched amine (HBPA) was synthesized and grafted to graphene oxide (GO), generating a hyper-branched amine-functionalized GO (FGO). A novel soy protein-based adhesive was developed by mixing FGO with soy protein (SPI) and a low dose polyamidoamine-epichlorohydrin (PAE). Results showed that the addition of only 0.4 wt% FGO and 0.75 wt% PAE to the SPI adhesive formulation enhanced the wet shear strength of plywood to 1.18 MPa, which was 181% higher than that of the adhesive without enhancement. The enhanced performance is attributed to the denser cross-linking structure and improved toughness of the adhesive layer. Using FGO in the adhesive formulation also greatly reduced the concentration of the additive cross-linker by up to 78.6% when compared with values reported in the literature. Thus, using a hyper-branched functionalized nano-material to form an organic\u2013inorganic hybrid structure is an effective and efficient strategy to reinforce the composites and polymers. It significantly reduces the chemical additive levels, and is a practical way to develop a sustainable product.<\/jats:p>","DOI":"10.3390\/nano13010203","type":"journal-article","created":{"date-parts":[[2023,1,3]],"date-time":"2023-01-03T02:05:53Z","timestamp":1672711553000},"page":"203","update-policy":"https:\/\/doi.org\/10.3390\/mdpi_crossmark_policy","source":"Crossref","is-referenced-by-count":18,"title":["Improving Bond Performance and Reducing Cross-Linker Dosage of Soy Protein Adhesive via Hyper-Branched and Organic\u2013Inorganic Hybrid Structures"],"prefix":"10.3390","volume":"13","author":[{"given":"Zheng","family":"Cui","sequence":"first","affiliation":[{"name":"MOE Key Laboratory of Wooden Material Science and Application & Beijing Key Laboratory of Wood Science and Engineering, Beijing Forestry University, Beijing 100083, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yecheng","family":"Xu","sequence":"additional","affiliation":[{"name":"MOE Key Laboratory of Wooden Material Science and Application & Beijing Key Laboratory of Wood Science and Engineering, Beijing Forestry University, Beijing 100083, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Gang","family":"Sun","sequence":"additional","affiliation":[{"name":"MOE Key Laboratory of Wooden Material Science and Application & Beijing Key Laboratory of Wood Science and Engineering, Beijing Forestry University, Beijing 100083, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Lai","family":"Peng","sequence":"additional","affiliation":[{"name":"Arte Mundi Group Co., Ltd., Shanghai 201700, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jianzhang","family":"Li","sequence":"additional","affiliation":[{"name":"MOE Key Laboratory of Wooden Material Science and Application & Beijing Key Laboratory of Wood Science and Engineering, Beijing Forestry University, Beijing 100083, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jing","family":"Luo","sequence":"additional","affiliation":[{"name":"College of Materials Science and Engineering, Nanjing Forestry University, Longpan Road 159, Xuanwu District, Nanjing 210037, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-7571-4903","authenticated-orcid":false,"given":"Qiang","family":"Gao","sequence":"additional","affiliation":[{"name":"MOE Key Laboratory of Wooden Material Science and Application & Beijing Key Laboratory of Wood Science and Engineering, Beijing Forestry University, Beijing 100083, China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"1968","published-online":{"date-parts":[[2023,1,2]]},"reference":[{"key":"ref_1","doi-asserted-by":"crossref","first-page":"2033","DOI":"10.1007\/s10924-020-02036-8","article-title":"Soy Protein Adhesives for Particleboard Production\u2014A Review","volume":"29","author":"Bacigalupe","year":"2021","journal-title":"J. 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