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this work, the simple fabrication of a new superhydrophobic magnetic sponge based on CNTs, NiFe2O4 nanoparticles, and PDMS was investigated. CNTs were synthesized by chemical vapor deposition (CVD) on a nickel ferrite catalyst supported on aluminum oxide (NiFe2O4\/Al2O3). The synthesis of nickel ferrite (NiFe) was accomplished using the sol\u2013gel method, yielding magnetic nanoparticles (43 Am2kg\u22121, coercivity of 93 Oe, 21\u201329 nm). A new superhydrophobic magnetic PU\/CNT\/NiFe2O4\/PDMS sponge was fabricated using a polyurethane (PU) sponge, CNTs, NiFe2O4 nanoparticles, and polydimethylsiloxane (PDMS) through the immersion coating method. The new PU\/CNT\/NiFe2O4\/PDMS sponge exhibits excellent superhydrophobic\/oleophilic\/mechanical properties and water repellency (water absorption rate of 0.4%) while having good absorption of oil, olive oil, and organic liquids of different densities (absorption capacity of 21.38 to 44.83 g\/g), excellent separation efficiency (up to 99.81%), the ability to be reused for removing oil and organic solvents for more than 10 cycles, and easy control and separation from water using a magnet. The new PU\/CNT\/NiFe2O4\/PDMS sponge is a promising candidate as a reusable sorbent for collecting oil and organic pollutants and can also be used as a hydrophobic filter due to its excellent mechanical properties.<\/jats:p>","DOI":"10.3390\/nano14231942","type":"journal-article","created":{"date-parts":[[2024,12,3]],"date-time":"2024-12-03T11:48:56Z","timestamp":1733226536000},"page":"1942","update-policy":"https:\/\/doi.org\/10.3390\/mdpi_crossmark_policy","source":"Crossref","is-referenced-by-count":13,"title":["Carbon-Nanotube-Based Superhydrophobic Magnetic Nanomaterial as Absorbent for Rapid and Efficient Oil\/Water Separation"],"prefix":"10.3390","volume":"14","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-0759-1539","authenticated-orcid":false,"given":"Rabiga M.","family":"Kudaibergenova","sequence":"first","affiliation":[{"name":"Department of Chemistry and Chemical Technology, Faculty of Technology, M. Kh. Dulaty Taraz University, 60 Tole Bi Street, Taraz 080000, Kazakhstan"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-5360-5298","authenticated-orcid":false,"given":"Fernanda F.","family":"Roman","sequence":"additional","affiliation":[{"name":"CIMO, LA SusTEC, Instituto Polit\u00e9cnico de Bragan\u00e7a, Campus de Santa Apol\u00f3nia, 5300-253 Bragan\u00e7a, Portugal"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-6795-2335","authenticated-orcid":false,"given":"Adriano S.","family":"Silva","sequence":"additional","affiliation":[{"name":"CIMO, LA SusTEC, Instituto Polit\u00e9cnico de Bragan\u00e7a, Campus de Santa Apol\u00f3nia, 5300-253 Bragan\u00e7a, Portugal"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Gulnar K.","family":"Sugurbekova","sequence":"additional","affiliation":[{"name":"Department of Chemistry, Faculty of Natural Sciences, Eurasian National University Named after L.N. 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