{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,9,20]],"date-time":"2026-09-20T07:57:28Z","timestamp":1789891048035,"version":"4.0.1"},"reference-count":332,"publisher":"MDPI AG","issue":"12","license":[{"start":{"date-parts":[[2026,6,11]],"date-time":"2026-06-11T00:00:00Z","timestamp":1781136000000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/creativecommons.org\/licenses\/by\/4.0\/"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"publisher","award":["22273016"],"award-info":[{"award-number":["22273016"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"publisher"}]},{"award":["22273016"],"award-info":[{"award-number":["22273016"]}],"id":[{"id":"https:\/\/ror.org\/01h0zpd94","id-type":"ROR","asserted-by":"publisher"}]},{"DOI":"10.13039\/501100006407","name":"Natural Science Foundation of Henan Province","doi-asserted-by":"publisher","award":["252300421043"],"award-info":[{"award-number":["252300421043"]}],"id":[{"id":"10.13039\/501100006407","id-type":"DOI","asserted-by":"publisher"}]},{"name":"Plan for Henan Province University Science and Technology Innovation Team","award":["25IRTSTHN002"],"award-info":[{"award-number":["25IRTSTHN002"]}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":["Nanomaterials"],"abstract":"<jats:p>The continuous rise in carbon emissions poses a serious threat to the global climate, driving the urgent need for efficient CCUS technologies. Ionic liquids (ILs), with their negligible vapor pressure, excellent thermal stability, and tunable molecular structures, have emerged as promising materials for CO2 capture. However, the high viscosity of bulk ILs severely restricts gas mass transfer. To overcome this limitation, integrating ILs with porous materials featuring large surface areas and well-defined pore structures has emerged as a synergistic strategy, combining the high CO2 affinity and selectivity of ILs with the rapid mass transfer and structural stability of porous supports. This review systematically summarizes the CO2 capture mechanisms and limitations of bulk ILs and further highlights recent advances in the design, synthesis, and applications of IL-based hybrid adsorbents. Particular attention is given to confinement-enhanced mechanisms, whereby nanoscale confinement fundamentally alters the physicochemical behavior of ILs, transforming them from disordered bulk liquids into ordered, interface-dominated systems. In addition, the life-cycle assessment and techno-economic analysis of IL hybrid systems are critically evaluated.<\/jats:p>","DOI":"10.3390\/nano16120727","type":"journal-article","created":{"date-parts":[[2026,6,17]],"date-time":"2026-06-17T05:56:31Z","timestamp":1781675791000},"page":"727","update-policy":"https:\/\/doi.org\/10.3390\/mdpi_crossmark_policy","source":"Crossref","is-referenced-by-count":2,"title":["Research Progress of Ionic Liquids Hybridized with Porous Materials for CO2 Capture: From Bulk to Confinement-Enhanced Adsorbents"],"prefix":"10.3390","volume":"16","author":[{"ORCID":"https:\/\/orcid.org\/0009-0007-2941-3748","authenticated-orcid":false,"given":"Enqi","family":"Zhang","sequence":"first","affiliation":[{"name":"Henan Key Laboratory of Green Chemistry, Collaborative Innovation Center of Henan Province for Green Manufacturing of Fine Chemicals, Key Laboratory of Green Chemical Media and Reactions, Ministry of Education, School of Chemistry and Chemical Engineering, Henan Normal University, Xinxiang 453007, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Zhenzhen","family":"Wang","sequence":"additional","affiliation":[{"name":"Henan Key Laboratory of Green Chemistry, Collaborative Innovation Center of Henan Province for Green Manufacturing of Fine Chemicals, Key Laboratory of Green Chemical Media and Reactions, Ministry of Education, School of Chemistry and Chemical Engineering, Henan Normal University, Xinxiang 453007, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yanwei","family":"Chi","sequence":"additional","affiliation":[{"name":"Henan Key Laboratory of Green Chemistry, Collaborative Innovation Center of Henan Province for Green Manufacturing of Fine Chemicals, Key Laboratory of Green Chemical Media and Reactions, Ministry of Education, School of Chemistry and Chemical Engineering, Henan Normal University, Xinxiang 453007, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-1865-864X","authenticated-orcid":false,"given":"Zhiyong","family":"Li","sequence":"additional","affiliation":[{"name":"Henan Key Laboratory of Green Chemistry, Collaborative Innovation Center of Henan Province for Green Manufacturing of Fine Chemicals, Key Laboratory of Green Chemical Media and Reactions, Ministry of Education, School of Chemistry and Chemical Engineering, Henan Normal University, Xinxiang 453007, China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"1968","published-online":{"date-parts":[[2026,6,11]]},"reference":[{"key":"ref_1","doi-asserted-by":"crossref","first-page":"1404","DOI":"10.1126\/science.abo3378","article-title":"Current global efforts are insufficient to limit warming to 1.5 \u00b0C","volume":"376","author":"Matthews","year":"2022","journal-title":"Science"},{"key":"ref_2","doi-asserted-by":"crossref","first-page":"eabo6849","DOI":"10.1126\/sciadv.abo6849","article-title":"A scalable solid-state nanoporous network with atomic-level interaction design for carbon dioxide capture","volume":"8","author":"Mao","year":"2022","journal-title":"Sci. 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