{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,6,26]],"date-time":"2026-06-26T19:35:42Z","timestamp":1782502542812,"version":"3.54.5"},"reference-count":112,"publisher":"MDPI AG","issue":"14","license":[{"start":{"date-parts":[[2023,7,19]],"date-time":"2023-07-19T00:00:00Z","timestamp":1689724800000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/creativecommons.org\/licenses\/by\/4.0\/"}],"funder":[{"name":"Heilongjiang Natural Science Foundation Joint Guidance Project of China","award":["LH2022E097"],"award-info":[{"award-number":["LH2022E097"]}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":["Polymers"],"abstract":"<jats:p>Polylactic acid (PLA) is a biodegradable polyester polymer that is produced from renewable resources, such as corn or other carbohydrate sources. However, its poor toughness limits its commercialization. PLA composites can meet the growing performance needs of various fields, but limited research has focused on their sustainable applications in sports. This paper reviews the latest research on PLA and its composites by describing the characteristics, production, degradation process, and the latest modification methods of PLA. Then, it discusses the inherent advantages of PLA composites and expounds on different biodegradable materials and their relationship with the properties of PLA composites. Finally, the importance and application prospects of PLA composites in the field of sports are emphasized. Although PLA composites mixed with natural biomass materials have not been mass produced, they are expected to be sustainable materials used in various industries because of their simple process, nontoxicity, biodegradability, and low cost.<\/jats:p>","DOI":"10.3390\/polym15143096","type":"journal-article","created":{"date-parts":[[2023,7,19]],"date-time":"2023-07-19T21:21:46Z","timestamp":1689801706000},"page":"3096","update-policy":"https:\/\/doi.org\/10.3390\/mdpi_crossmark_policy","source":"Crossref","is-referenced-by-count":185,"title":["Biodegradable Polylactic Acid and Its Composites: Characteristics, Processing, and Sustainable Applications in Sports"],"prefix":"10.3390","volume":"15","author":[{"given":"Yueting","family":"Wu","sequence":"first","affiliation":[{"name":"Graduate School, College of Sports and Human Sciences, Post-Doctoral Mobile Research Station, Harbin Sport University, Harbin 150008, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Xing","family":"Gao","sequence":"additional","affiliation":[{"name":"Graduate School, College of Sports and Human Sciences, Post-Doctoral Mobile Research Station, Harbin Sport University, Harbin 150008, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Jie","family":"Wu","sequence":"additional","affiliation":[{"name":"Graduate School, College of Sports and Human Sciences, Post-Doctoral Mobile Research Station, Harbin Sport University, Harbin 150008, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Tongxi","family":"Zhou","sequence":"additional","affiliation":[{"name":"Graduate School, College of Sports and Human Sciences, Post-Doctoral Mobile Research Station, Harbin Sport University, Harbin 150008, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Tat Thang","family":"Nguyen","sequence":"additional","affiliation":[{"name":"College of Wood Industry and Interior Design, Vietnam National University of Forestry, Xuan Mai, Hanoi 13417, Vietnam"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Yutong","family":"Wang","sequence":"additional","affiliation":[{"name":"Graduate School, College of Sports and Human Sciences, Post-Doctoral Mobile Research Station, Harbin Sport University, Harbin 150008, China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"1968","published-online":{"date-parts":[[2023,7,19]]},"reference":[{"key":"ref_1","doi-asserted-by":"crossref","first-page":"129954","DOI":"10.1016\/j.molstruc.2021.129954","article-title":"Recent trends on bioplastics synthesis and characterizations: Polylactic acid (PLA) incorporated with tapioca starch for packaging applications","volume":"1232","author":"Yusoff","year":"2021","journal-title":"J. Mol. Struct."},{"key":"ref_2","doi-asserted-by":"crossref","first-page":"759","DOI":"10.1016\/j.cej.2017.07.068","article-title":"Complete stereo-complexation of enantiomeric polylactides for scalable continuous production","volume":"328","author":"Pan","year":"2017","journal-title":"Chem. Eng. J."},{"key":"ref_3","doi-asserted-by":"crossref","first-page":"4461","DOI":"10.1007\/s10570-017-1431-6","article-title":"Cellulose nanocrystals\/polyethylene glycol as bifunctional reinforcing\/compatibilizing agents in poly(lactic acid) nanofibers for controlling long-term in vitro drug release","volume":"24","author":"Yu","year":"2017","journal-title":"Cellulose"},{"key":"ref_4","doi-asserted-by":"crossref","unstructured":"Yang, C., Vora, H.D., and Chang, Y.B. (2016, January 11\u201317). Evaluation of auxetic polymeric structures for use in protective pads. Proceedings of the ASME International Mechanical Engineering Congress and Exposition (IMECE2016), Phoenix, AZ, USA.","DOI":"10.1115\/IMECE2016-67588"},{"key":"ref_5","doi-asserted-by":"crossref","unstructured":"Bartolucci, L., Cordiner, S., De Maina, E., Kumar, G., Mele, P., Mulone, V., Igli\u0144ski, B., and Piechota, G. (2023). Sustainable Valorization of Bioplastic Waste: A Review on Effective Recycling Routes for the Most Widely Used Biopolymers. Int. J. Mol. Sci., 24.","DOI":"10.3390\/ijms24097696"},{"key":"ref_6","doi-asserted-by":"crossref","first-page":"17151","DOI":"10.1039\/D1RA02390J","article-title":"Poly(lactic acid) (PLA) and polyhydroxyalkanoates (PHAs), green alternatives to petroleum-based plastics: A review","volume":"11","author":"Naser","year":"2021","journal-title":"RSC Adv."},{"key":"ref_7","first-page":"13","article-title":"Bioplastics: Their advantages and concerns","volume":"11","author":"Sarkingobir","year":"2021","journal-title":"Mater. Metallurg. Eng."},{"key":"ref_8","doi-asserted-by":"crossref","unstructured":"Naser, A.Z., Deiab, I., Defersha, F., and Yang, S. (2021). Expanding poly(lactic acid) (PLA) and polyhydroxyalkanoates (PHAs) applications: A review on modifications and effects. Polymers, 13.","DOI":"10.3390\/polym13234271"},{"key":"ref_9","doi-asserted-by":"crossref","unstructured":"Rezvani, G.E., Khosravi, F., Saedi, A.A., Dai, Y., Neisiany, R.E., Foroughi, F., Wu, M., Das, O., and Ramakrishna, S. (2021). The Life Cycle Assessment for Polylactic Acid (PLA) to Make It a Low-Carbon Material. Polymers, 13.","DOI":"10.3390\/polym13111854"},{"key":"ref_10","unstructured":"(2023, May 21). European Bioplastics. Bioplastics: Facts and Figures. Available online: https:\/\/www.european-bioplastics.org\/bioplastics-facts-figures\/."},{"key":"ref_11","doi-asserted-by":"crossref","first-page":"1","DOI":"10.1080\/15583720701834133","article-title":"Polymers from Renewable Resources: A Perspective for a Special Issue of Polymer Reviews","volume":"48","author":"Williams","year":"2008","journal-title":"Polym. Rev."},{"key":"ref_12","doi-asserted-by":"crossref","first-page":"47","DOI":"10.1016\/j.polymer.2018.02.032","article-title":"Disentanglement induced by uniaxial pre-stretching as a key factor for toughening poly((L)-lactic acid) sheets","volume":"140","author":"Chen","year":"2018","journal-title":"Polymer"},{"key":"ref_13","doi-asserted-by":"crossref","first-page":"100548","DOI":"10.1016\/j.coco.2020.100548","article-title":"Recent progress on chemical modification of cellulose for high mechanical-performance poly(lactic acid)\/cellulose composite: A review","volume":"23","author":"Zhou","year":"2021","journal-title":"Compos. Commun."},{"key":"ref_14","unstructured":"Henton, D.E., Gruber, P., Lunt, J., and Randall, J. (2005). Natural Fibers, Biopolymers, and Biocomposites, CRC Press."},{"key":"ref_15","doi-asserted-by":"crossref","first-page":"1","DOI":"10.1016\/j.compositesb.2017.11.048","article-title":"PLA based biocomposites reinforced with Posidonia oceanica leaves","volume":"139","author":"Scaffaro","year":"2018","journal-title":"Compos. Part B Eng."},{"key":"ref_16","doi-asserted-by":"crossref","first-page":"1657","DOI":"10.1016\/j.progpolymsci.2012.07.005","article-title":"Poly(lactic acid) crystallization","volume":"37","author":"Saeidlou","year":"2012","journal-title":"Prog. Polym. Sci."},{"key":"ref_17","doi-asserted-by":"crossref","first-page":"287","DOI":"10.1016\/j.compositesb.2018.10.078","article-title":"Improvement of thermal behaviors of biodegradable poly(lactic acid) polymer: A review","volume":"164","author":"Jin","year":"2019","journal-title":"Compos. Part B Eng."},{"key":"ref_18","doi-asserted-by":"crossref","first-page":"77","DOI":"10.1016\/j.polymdegradstab.2017.05.016","article-title":"Synthesis of meso-lactide by thermal configurational inversion and depolymerization of poly(l-lactide) and thermal configurational inversion of lactides","volume":"141","author":"Tsuji","year":"2017","journal-title":"Polym. Degrad. Stab."},{"key":"ref_19","doi-asserted-by":"crossref","first-page":"145","DOI":"10.1016\/S0141-3910(97)00148-1","article-title":"Large-scale production, properties and commercial applications of polylactic acid polymers","volume":"59","author":"Lunt","year":"1998","journal-title":"Polym. Degrad. Stab."},{"key":"ref_20","doi-asserted-by":"crossref","first-page":"3116","DOI":"10.1007\/s10924-020-01840-6","article-title":"Packaging Film of PP\/LDPE\/PLA\/Clay Composite: Physical, Barrier and Degradable Properties","volume":"28","author":"Mooninta","year":"2020","journal-title":"J. Polym. Environ."},{"key":"ref_21","doi-asserted-by":"crossref","first-page":"4269792","DOI":"10.1155\/2020\/4269792","article-title":"Study on Thermal Behavior of Some Biocompatible and Biodegradable Materials Based on Plasticized PLA, Chitosan, and Rosemary Ethanolic Extract","volume":"2020","author":"Vasile","year":"2020","journal-title":"Int. J. Polym. Sci."},{"key":"ref_22","doi-asserted-by":"crossref","first-page":"535","DOI":"10.1016\/j.polymdegradstab.2004.10.011","article-title":"Polylactide\/montmorillonite nanocomposites: Study of the hydrolytic degradation","volume":"87","author":"Paul","year":"2005","journal-title":"Polym. Degrad. Stab."},{"key":"ref_23","doi-asserted-by":"crossref","first-page":"4483","DOI":"10.1016\/S0142-9612(02)00168-0","article-title":"A novel porous cells scaffold made of polylactide\u2013dextran blend by combining phase-separation and particle-leaching techniques","volume":"23","author":"Cai","year":"2002","journal-title":"Biomaterials"},{"key":"ref_24","doi-asserted-by":"crossref","first-page":"2885","DOI":"10.21817\/ijet\/2017\/v9i4\/170904066","article-title":"Mathematical Modelling & Pressure Drop Analysis of Fused Deposition Modelling Feed Wire","volume":"9","author":"Haleem","year":"2017","journal-title":"Int. J. Eng. Technol."},{"key":"ref_25","doi-asserted-by":"crossref","first-page":"367","DOI":"10.1016\/j.addr.2016.06.012","article-title":"Physical and mechanical properties of PLA, and their functions in widespread appli-cations\u2014A comprehensive review","volume":"107","author":"Farah","year":"2016","journal-title":"Adv. Drug Deliv. Rev."},{"key":"ref_26","doi-asserted-by":"crossref","first-page":"192","DOI":"10.1016\/j.addr.2016.07.004","article-title":"Poly(lactic acid) based hydrogels","volume":"107","author":"Basu","year":"2016","journal-title":"Adv. Drug Deliv. Rev."},{"key":"ref_27","doi-asserted-by":"crossref","first-page":"1402","DOI":"10.1016\/j.proeng.2012.07.534","article-title":"Poly (Lactic Acid) Production for Tissue Engineering Applications","volume":"42","author":"Lopes","year":"2012","journal-title":"Procedia Eng."},{"key":"ref_28","doi-asserted-by":"crossref","first-page":"1123","DOI":"10.1016\/S0079-6700(02)00012-6","article-title":"Properties of lactic acid based polymers and their correlation with composition","volume":"27","author":"Stolt","year":"2002","journal-title":"Prog. Polym. Sci."},{"key":"ref_29","doi-asserted-by":"crossref","first-page":"7541","DOI":"10.1016\/S0032-3861(01)00150-1","article-title":"Synthesis of polylactides in the presence of coinitiators with different numbers of hydroxyl groups","volume":"42","author":"Korhonen","year":"2001","journal-title":"Polymer"},{"key":"ref_30","doi-asserted-by":"crossref","first-page":"2061","DOI":"10.1002\/pen.25511","article-title":"A review on degradation mechanisms of polylactic acid: Hydrolytic, photodegradative, microbial, and enzymatic degradation","volume":"60","author":"Zaaba","year":"2020","journal-title":"Polym. Eng. Sci."},{"key":"ref_31","doi-asserted-by":"crossref","first-page":"1713","DOI":"10.1007\/s10118-015-1715-y","article-title":"The stereocomplex formation and phase separation of PLLA\/PDLA blends with different optical purities and molecular weights","volume":"33","author":"Shao","year":"2015","journal-title":"Chin. J. Polym. Sci."},{"key":"ref_32","doi-asserted-by":"crossref","first-page":"17","DOI":"10.1016\/j.addr.2016.04.003","article-title":"PLA composites: From production to properties","volume":"107","author":"Murariu","year":"2016","journal-title":"Adv. Drug Deliv. Rev."},{"key":"ref_33","doi-asserted-by":"crossref","first-page":"468","DOI":"10.1016\/j.eurpolymj.2005.07.022","article-title":"Synthesis of high-molecular-weight poly(l-lactic acid) through the direct condensation polymerization of l-lactic acid in bulk state","volume":"42","author":"Chen","year":"2006","journal-title":"Eur. Polym. J."},{"key":"ref_34","doi-asserted-by":"crossref","unstructured":"Huang, S., Xue, Y., Yu, B., Wang, L., Zhou, C., and Ma, Y. (2021). A Review of the Recent Developments in the Bioproduction of Polylactic Acid and Its Precursors Optically Pure Lactic Acids. Molecules, 26.","DOI":"10.3390\/molecules26216446"},{"key":"ref_35","doi-asserted-by":"crossref","first-page":"238","DOI":"10.1016\/j.rser.2019.03.050","article-title":"Towards sustainability of lactic acid and poly-lactic acid polymers production","volume":"108","author":"Pejin","year":"2019","journal-title":"Renew. Sustain. Energy Rev."},{"key":"ref_36","doi-asserted-by":"crossref","unstructured":"Kalia, S., and Av\u00e9rous, L. (2011). Biopolymers: Biomedical and Environmental Applications, John Wiley & Sons.","DOI":"10.1002\/9781118164792"},{"key":"ref_37","doi-asserted-by":"crossref","first-page":"122091","DOI":"10.1016\/j.polymer.2019.122091","article-title":"Structuring poly (lactic acid) film with excellent tensile toughness through extrusion blow molding","volume":"187","author":"Zengwen","year":"2020","journal-title":"Polymer"},{"key":"ref_38","doi-asserted-by":"crossref","first-page":"73","DOI":"10.37358\/MP.17.1.4789","article-title":"Influence of plasticizers over some physico-chemical properties of PLA","volume":"54","author":"Rapa","year":"2017","journal-title":"Mater. Plast."},{"key":"ref_39","doi-asserted-by":"crossref","first-page":"41","DOI":"10.1016\/j.tca.2015.05.019","article-title":"Dynamic mechanical properties of PLA\/PHBV, PLA\/PCL, PHBV\/PCL blends and their nano-composites with TiO2 as nanofiller","volume":"613","author":"Mofokeng","year":"2015","journal-title":"Thermochim. Acta"},{"key":"ref_40","doi-asserted-by":"crossref","first-page":"121728","DOI":"10.1016\/j.polymer.2019.121728","article-title":"Transform poly (lactic acid) packaging film from brittleness to toughness using traditional industrial equipments","volume":"180","author":"Cao","year":"2019","journal-title":"Polymer"},{"key":"ref_41","doi-asserted-by":"crossref","first-page":"163","DOI":"10.1016\/j.tca.2010.08.009","article-title":"Detail kinetic analysis of the thermal decomposition of PLA with oxidized multi-walled carbon nanotubes","volume":"511","author":"Chrissafis","year":"2010","journal-title":"Thermochim. Acta"},{"key":"ref_42","doi-asserted-by":"crossref","first-page":"61","DOI":"10.1016\/j.compositesb.2012.10.013","article-title":"Covalent grafting of carbon nanotubes to PLA in order to improve compatibility","volume":"46","author":"Seligra","year":"2013","journal-title":"Compos. Part B Eng."},{"key":"ref_43","doi-asserted-by":"crossref","first-page":"1200","DOI":"10.1002\/jbm.b.33670","article-title":"Synthesis and wound healing of alternating block polyurethanes based on poly(lactic acid) (PLA) and poly(ethylene glycol) (PEG)","volume":"105","author":"Li","year":"2017","journal-title":"J. Biomed. Mater. Res. Part B Appl. Biomater."},{"key":"ref_44","doi-asserted-by":"crossref","first-page":"e202202660","DOI":"10.1002\/anie.202202660","article-title":"Electrochemically Controlled Switchable Copolymerization of Lactide, Carbon Dioxide, and Epoxides","volume":"61","author":"Huang","year":"2022","journal-title":"Angew. Chem. Int. Ed."},{"key":"ref_45","doi-asserted-by":"crossref","first-page":"377","DOI":"10.1016\/j.resconrec.2005.08.006","article-title":"Economics and GHG emission reduction of a PLA bio-refinery system\u2014Combining bottom-up analysis with price elasticity effects","volume":"46","author":"Dornburg","year":"2006","journal-title":"Resour. Conserv. Recycl."},{"key":"ref_46","doi-asserted-by":"crossref","first-page":"1720","DOI":"10.1016\/j.progpolymsci.2013.05.010","article-title":"Multifunctional nanostructured PLA materials for packaging and tissue engineering","volume":"38","author":"Armentano","year":"2013","journal-title":"Prog. Polym. Sci."},{"key":"ref_47","doi-asserted-by":"crossref","unstructured":"McKeown, P., and Jones, M.D. (2020). The Chemical Recycling of PLA: A Review. Sustain. Chem., 1.","DOI":"10.3390\/suschem1010001"},{"key":"ref_48","doi-asserted-by":"crossref","first-page":"313","DOI":"10.1007\/s10924-012-0547-x","article-title":"Kinetics of Hydrolytic Degradation of PLA","volume":"21","author":"Piemonte","year":"2013","journal-title":"J. Polym. Environ."},{"key":"ref_49","doi-asserted-by":"crossref","first-page":"1504","DOI":"10.1016\/j.progpolymsci.2013.05.014","article-title":"Polylactide (PLA)-based nanocomposites","volume":"38","author":"Raquez","year":"2013","journal-title":"Prog. Polym. Sci."},{"key":"ref_50","doi-asserted-by":"crossref","first-page":"e53477","DOI":"10.1002\/app.53477","article-title":"A review of research and application of polylactic acid composites","volume":"140","author":"Li","year":"2022","journal-title":"J. Appl. Polym. Sci."},{"key":"ref_51","doi-asserted-by":"crossref","first-page":"930","DOI":"10.1016\/j.ijbiomac.2022.07.140","article-title":"Recent advances in 3D-printed polylactide and polycaprolactone-based biomaterials for tissue engineering applications","volume":"218","author":"Arif","year":"2022","journal-title":"Int. J. Biol. Macromol."},{"key":"ref_52","doi-asserted-by":"crossref","first-page":"19","DOI":"10.1016\/j.compositesb.2016.02.032","article-title":"Influence of fiber modifications on PLA\/fiber composites. Behavior to accelerated weathering","volume":"92","author":"Spiridon","year":"2016","journal-title":"Compos. Part B Eng."},{"key":"ref_53","doi-asserted-by":"crossref","first-page":"4856","DOI":"10.1002\/app.24829","article-title":"Wood-fiber-reinforced poly(lactic acid) composites: Evaluation of the physicomechanical and morphological properties","volume":"102","author":"Huda","year":"2006","journal-title":"J. Appl. Polym. Sci."},{"key":"ref_54","doi-asserted-by":"crossref","first-page":"1026","DOI":"10.1016\/j.compositesb.2007.11.009","article-title":"A potential material for tissue engineering: Silkworm silk\/PLA biocomposite","volume":"39","author":"Cheung","year":"2008","journal-title":"Compos. Part B Eng."},{"key":"ref_55","doi-asserted-by":"crossref","unstructured":"Hongdilokkul, P., Keeratipinit, K., Chawthai, S., Hararak, B., Seadan, M., and Suttiruengwong, S. (2015, January 16\u201319). A study on properties of PLA\/PBAT from blown film process. Proceedings of the Global Conference on Polymer and Composite Materials (PCM), Beijing, China.","DOI":"10.1088\/1757-899X\/87\/1\/012112"},{"key":"ref_56","doi-asserted-by":"crossref","unstructured":"Injorhor, P., Trongsatitkul, T., Wittayakun, J., Ruksakulpiwat, C., and Ruksakulpiwat, Y. (2023). Biodegradable polylactic acid-polyhydroxyalkanoate-based nanocomposites with bio-hydroxyapatite: Preparation and characterization. Polymers, 15.","DOI":"10.3390\/polym15051261"},{"key":"ref_57","doi-asserted-by":"crossref","first-page":"118298","DOI":"10.1016\/j.apcata.2021.118298","article-title":"Catalytic fast pyrolysis of beech wood lignin isolated by different biomass (pre) treatment processes: Organosolv, hydrothermal and enzymatic hydrolysis","volume":"623","author":"Margellou","year":"2021","journal-title":"Appl. Catal. A-Gen."},{"key":"ref_58","doi-asserted-by":"crossref","first-page":"107","DOI":"10.1080\/15583724.2014.971124","article-title":"A Review of Natural Fibers Used in Biocomposites: Plant, Animal and Regenerated Cellulose Fibers","volume":"55","author":"Ramamoorthy","year":"2015","journal-title":"Polym. Rev."},{"key":"ref_59","doi-asserted-by":"crossref","unstructured":"Sanivada, U.K., Marmol, G., Brito, F.P., and Fangueiro, R. (2020). PLA composites reinforced with flax and jute fibers\u2014A review of recent trends, processing parameters and mechanical properties. Polymers, 12.","DOI":"10.3390\/polym12102373"},{"key":"ref_60","doi-asserted-by":"crossref","first-page":"362","DOI":"10.1080\/15583724.2015.1108334","article-title":"Dynamic Mechanical Thermal Analysis of Polymer Composites Reinforced with Natural Fibers","volume":"56","author":"Costa","year":"2016","journal-title":"Polym. Rev."},{"key":"ref_61","doi-asserted-by":"crossref","first-page":"e05486","DOI":"10.1016\/j.heliyon.2020.e05486","article-title":"Preparation and characterization of cellulose nanocrystal extracted from ramie fibers by sulfuric acid hydrolysis","volume":"6","author":"Kusmono","year":"2020","journal-title":"Heliyon"},{"key":"ref_62","doi-asserted-by":"crossref","first-page":"220","DOI":"10.1016\/j.mattod.2013.06.004","article-title":"Nanocellulose: A new ageless bionanomaterial","volume":"16","author":"Dufresne","year":"2013","journal-title":"Mater. Today"},{"key":"ref_63","doi-asserted-by":"crossref","first-page":"6365","DOI":"10.1021\/ma00122a053","article-title":"Polymer Nanocomposites Reinforced by Cellulose Whiskers","volume":"28","author":"Favier","year":"1995","journal-title":"Macromolecules"},{"key":"ref_64","doi-asserted-by":"crossref","first-page":"301","DOI":"10.1016\/j.carbpol.2012.05.042","article-title":"Mechanical properties and in vitro degradation of electrospun bio-nanocomposite mats from PLA and cellulose nanocrystals","volume":"90","author":"Shi","year":"2012","journal-title":"Carbohydr. Polym."},{"key":"ref_65","doi-asserted-by":"crossref","first-page":"4843","DOI":"10.1177\/09544062211055662","article-title":"Fabrication techniques of polymeric nanocomposites: A comprehensive review","volume":"236","author":"Kamal","year":"2022","journal-title":"Proc. Inst. Mech. Eng. Part C J. Mech. Eng. Sci."},{"key":"ref_66","doi-asserted-by":"crossref","first-page":"204","DOI":"10.1016\/j.compositesa.2018.08.025","article-title":"Water vapor and oxygen barrier properties of extrusion-blown poly(lactic acid)\/cellulose nanocrystals nanocomposite films","volume":"114","author":"Karkhanis","year":"2018","journal-title":"Compos. Part A-Appl. Sci. Manuf."},{"key":"ref_67","doi-asserted-by":"crossref","first-page":"106458","DOI":"10.1016\/j.polymertesting.2020.106458","article-title":"Cellulose nanocrystals as biobased nucleation agents in poly-l-lactide scaffold: Crystallization behavior and mechanical properties","volume":"85","author":"Shuai","year":"2020","journal-title":"Polym. Test."},{"key":"ref_68","doi-asserted-by":"crossref","unstructured":"Beluns, S., Platnieks, O., Gaidukovs, S., Starkova, O., Sabalina, A., Grase, L., Thakur, V.K., and Gaidukova, G. (2021). Lignin and Xylan as Interface Engineering Additives for Improved Environmental Durability of Sustainable Cellulose Nanopapers. Int. J. Mol. Sci., 22.","DOI":"10.3390\/ijms222312939"},{"key":"ref_69","doi-asserted-by":"crossref","first-page":"43596","DOI":"10.1038\/srep43596","article-title":"All Biomass and UV Protective Composite Composed of Compatibilized Lignin and Poly (Lactic-acid)","volume":"7","author":"Kim","year":"2017","journal-title":"Sci. Rep."},{"key":"ref_70","doi-asserted-by":"crossref","first-page":"1072","DOI":"10.1021\/sc500087z","article-title":"Progress in green polymer composites from lignin for multi-functional applications: A review","volume":"2","author":"Thakur","year":"2014","journal-title":"ACS Sustain. Chem. Eng."},{"key":"ref_71","doi-asserted-by":"crossref","first-page":"855","DOI":"10.1016\/j.ijbiomac.2018.03.140","article-title":"Design, characterization and preliminary biological evaluation of new lignin-PLA biocomposites","volume":"114","author":"Spiridon","year":"2018","journal-title":"Int. J. Biol. Macromol."},{"key":"ref_72","doi-asserted-by":"crossref","unstructured":"Tanase-Opedal, M., Espinosa, E., Rodriguez, A., and Chinga-Carrasco, G. (2019). Lignin: A Biopolymer from forestry biomass for bio-composites and 3D Printing. Materials, 12.","DOI":"10.3390\/ma12183006"},{"key":"ref_73","doi-asserted-by":"crossref","first-page":"173","DOI":"10.1016\/j.compscitech.2014.07.015","article-title":"Can silk become an effective reinforcing fibre? A property comparison with flax and glass reinforced composites","volume":"101","author":"Shah","year":"2014","journal-title":"Compos. Sci. Technol."},{"key":"ref_74","doi-asserted-by":"crossref","unstructured":"Luzi, F., Puglia, D., and Torre, L. (2019). Natural Fiber Biodegradable Composites and Nanocomposites: A Biomedical Application, Woodhead Publishing Ltd.","DOI":"10.1016\/B978-0-08-102426-3.00010-2"},{"key":"ref_75","doi-asserted-by":"crossref","first-page":"1978","DOI":"10.1016\/j.polymdegradstab.2010.07.015","article-title":"Silkworm silk\/poly(lactic acid) biocomposites: Dynamic mechanical, thermal and biodegradable properties","volume":"95","author":"Zhao","year":"2010","journal-title":"Polym. Degrad. Stab."},{"key":"ref_76","unstructured":"Cheung, H.Y., Dean, J., Stearn, B., and Clyne, T.W. (2012, January 24\u201328). Characterisation on PLA\u2013silk fibre composites for prosthetic applications. Proceedings of the 15th European Conference on Composite Materials, Venice, Italy."},{"key":"ref_77","doi-asserted-by":"crossref","first-page":"3064","DOI":"10.1021\/acsbiomaterials.6b00279","article-title":"Influence of Hydroxyl Groups on the Cell Viability of Polyhydroxyalkanoate (PHA) Scaffolds for Tissue Engineering","volume":"3","author":"Insomphun","year":"2017","journal-title":"ACS Biomater. Sci. Eng."},{"key":"ref_78","doi-asserted-by":"crossref","first-page":"193","DOI":"10.1177\/8756087906067324","article-title":"Studies toward producing eco-friendly plastics","volume":"22","author":"Khare","year":"2006","journal-title":"J. Plast Film Sheet."},{"key":"ref_79","doi-asserted-by":"crossref","unstructured":"Sun, J.Y., Shen, J.J., Chen, S.K., Cooper, M.A., Fu, H.B., Wu, D.M., and Yang, Z.G. (2018). Nanofiller Reinforced Biodegradable PLA\/PHA Composites: Current Status and Future Trends. Polymers, 10.","DOI":"10.3390\/polym10050505"},{"key":"ref_80","unstructured":"Lee, C.H., Sapuan, S.M., Ilyas, R.A., Lee, S.H., and Khalina, A. (2020). Advanced Processing, Properties, and Applications of Starch and Other Bio-Based Polymers, Elsevier."},{"key":"ref_81","doi-asserted-by":"crossref","first-page":"842","DOI":"10.1016\/j.polymertesting.2013.04.004","article-title":"A study of morphological, thermal, rheo-logical and barrier properties of Poly (3-hydroxybutyrate-Co-3-Hydroxyvalerate)\/polylactide blends prepared by melt mixing","volume":"32","author":"Zembouai","year":"2013","journal-title":"Polym. Test"},{"key":"ref_82","doi-asserted-by":"crossref","first-page":"2363","DOI":"10.1002\/app.20734","article-title":"Morphologies and mechanical properties of polylactide blends with medium chain length poly(3-hydroxyalkanoate) and chemically modified poly(3-hydroxyalkanoate)","volume":"93","author":"Takagi","year":"2004","journal-title":"J. Appl. Polym. Sci."},{"key":"ref_83","doi-asserted-by":"crossref","unstructured":"Su, S. (2021). Prediction of the Miscibility of PBAT\/PLA Blends. Polymers, 13.","DOI":"10.3390\/polym13142339"},{"key":"ref_84","doi-asserted-by":"crossref","first-page":"59082","DOI":"10.1039\/C5RA10241C","article-title":"Phosphonium ionic liquids as new compatibilizing agents of biopolymer blends composed of poly(butylene-adipate-co-terephtalate)\/poly(lactic acid) (PBAT\/PLA)","volume":"5","author":"Lins","year":"2015","journal-title":"RSC Adv."},{"key":"ref_85","doi-asserted-by":"crossref","first-page":"109455","DOI":"10.1016\/j.polymdegradstab.2020.109455","article-title":"Effect of chain extender and light stabilizer on the weathering resistance of PBAT\/PLA blend films prepared by extrusion blowing","volume":"183","author":"Zhang","year":"2021","journal-title":"Polym. Degrad. Stab."},{"key":"ref_86","doi-asserted-by":"crossref","first-page":"27","DOI":"10.1016\/j.polymertesting.2015.02.005","article-title":"Influence of chain extender on mechanical, thermal and morpho-logical properties of blown films of PLA\/PBAT blends","volume":"43","author":"Arruda","year":"2015","journal-title":"Polym. Test"},{"key":"ref_87","doi-asserted-by":"crossref","first-page":"485","DOI":"10.1002\/pen.760270702","article-title":"The nucleation of microcellular thermoplastic foam with additives: Part I: Theoretical considerations","volume":"27","author":"Colton","year":"1987","journal-title":"Polym. Eng. Sci."},{"key":"ref_88","doi-asserted-by":"crossref","first-page":"187","DOI":"10.1002\/masy.200351122","article-title":"Impact of microcellular plastics on industrial practice and academic research","volume":"201","author":"Suh","year":"2003","journal-title":"Macromol. Symp."},{"key":"ref_89","doi-asserted-by":"crossref","first-page":"500","DOI":"10.1002\/pen.760270704","article-title":"Nucleation of microcellular foam: Theory and practice","volume":"27","author":"Colton","year":"1987","journal-title":"Polym. Eng. Sci."},{"key":"ref_90","doi-asserted-by":"crossref","first-page":"493","DOI":"10.1002\/pen.760270703","article-title":"The nucleation of microcellular thermoplastic foam with additives: Part II: Experimental results and dis-cussion","volume":"27","author":"Colton","year":"1987","journal-title":"Polym. Eng. Sci."},{"key":"ref_91","doi-asserted-by":"crossref","unstructured":"Ding, Y., Hassan, M.H., Bakker, O., Hinduja, S., and B\u00e1rtolo, P. (2021). A Review on Microcellular Injection Moulding. Materials, 14.","DOI":"10.3390\/ma14154209"},{"key":"ref_92","doi-asserted-by":"crossref","first-page":"500","DOI":"10.1016\/j.eurpolymj.2015.11.001","article-title":"Microcellular to nanocellular polymer foams: Progress (2004\u20132015) and future directions\u2013A review","volume":"73","author":"Okolieocha","year":"2015","journal-title":"Eur. Polym. J."},{"key":"ref_93","doi-asserted-by":"crossref","first-page":"210","DOI":"10.1016\/S0921-5093(00)01373-3","article-title":"Semi-solid processing of engineering alloys by a twin-screw rheomoulding process","volume":"299","author":"Ji","year":"2001","journal-title":"Mater. Sci. Eng. A"},{"key":"ref_94","doi-asserted-by":"crossref","unstructured":"Li, S., Jones, D.S., and Andrews, G.P. (2013). Hot Melt Extrusion: A Process Overview and Use in Manufacturing Solid Dispersions of Poorly Water-Soluble Drugs, Wiley.","DOI":"10.1002\/9781118444726.ch11"},{"key":"ref_95","doi-asserted-by":"crossref","first-page":"123872","DOI":"10.1016\/j.polymer.2021.123872","article-title":"Evolution of ordered structure of TPU in high-elastic state and their influences on the autoclave foaming of TPU and inter-bead bonding of expanded TPU beads","volume":"228","author":"Jiang","year":"2021","journal-title":"Polymer"},{"key":"ref_96","unstructured":"Tatara, R.A. (2017). Applied Plastics Engineering Handbook, Elsevier."},{"key":"ref_97","doi-asserted-by":"crossref","first-page":"1286","DOI":"10.1016\/j.promfg.2019.06.089","article-title":"An Overview on 3D Printing Technology: Technological, Materials, and Applications","volume":"35","author":"Shahrubudin","year":"2019","journal-title":"Procedia Manuf."},{"key":"ref_98","doi-asserted-by":"crossref","first-page":"172001","DOI":"10.1088\/1361-6528\/ab5f29","article-title":"3D printed nanomaterial-based electronic, biomedical, and bioelectronic devices","volume":"31","author":"Hales","year":"2020","journal-title":"Nanotechnology"},{"key":"ref_99","doi-asserted-by":"crossref","first-page":"1004","DOI":"10.1002\/adfm.201503316","article-title":"Inkjet-Printed Flexible Gold Electrode Arrays for Bioelectronic Interfaces","volume":"26","author":"Khan","year":"2016","journal-title":"Adv. Funct. Mater."},{"key":"ref_100","doi-asserted-by":"crossref","unstructured":"Morales, A.P., Guemes, A., Fernandez-Lopez, A., Valero, V.C., and Llano, S.D. (2017). Bamboo-polylactic acid (PLA) composite material for structural applications. Materials, 10.","DOI":"10.3390\/ma10111286"},{"key":"ref_101","doi-asserted-by":"crossref","first-page":"761","DOI":"10.1016\/j.compositesb.2019.01.057","article-title":"Multilayer cotton fabric bio-composites based on PLA and PHB co-polymer for industrial load carrying applications","volume":"163","author":"Battegazzore","year":"2019","journal-title":"Compos. Part B-Eng."},{"key":"ref_102","doi-asserted-by":"crossref","first-page":"405","DOI":"10.1177\/1528083714555779","article-title":"Development of cot-ton-rich\/polylactic acid fiber blend knitted fabrics for sports textiles","volume":"45","author":"Guruprasad","year":"2015","journal-title":"J. Ind. Text"},{"key":"ref_103","unstructured":"Raykar, S.J., Narke, M.M., Desai, S.B., and Warke, S.S. (2018). Techno-Societal 2018: Proceedings of the 2nd International Conference on Advanced Technologies for Societal Applications-Volume 2, Springer."},{"key":"ref_104","doi-asserted-by":"crossref","first-page":"025012","DOI":"10.1088\/1361-665X\/aaa3cf","article-title":"Behavior of auxetic structures under compression and impact forces","volume":"27","author":"Yang","year":"2018","journal-title":"Smart Mater. Struct."},{"key":"ref_105","doi-asserted-by":"crossref","unstructured":"Soltani, A., Noroozi, R., Bodaghi, M., Zolfagharian, A., and Hedayati, R. (2020). 3D Printing On-Water Sports Boards with Bio-Inspired Core Designs. Polymers, 12.","DOI":"10.3390\/polym12010250"},{"key":"ref_106","doi-asserted-by":"crossref","unstructured":"Kim, G.-J., Lee, K.-J., Choi, J.-W., and An, J.H. (2022). Modified Industrial Three-Dimensional Polylactic Acid Scaffold Cell Chip Promotes the Proliferation and Differentiation of Human Neural Stem Cells. Int. J. Mol. Sci., 23.","DOI":"10.3390\/ijms23042204"},{"key":"ref_107","doi-asserted-by":"crossref","unstructured":"Chen, C.H., Cheng, Y.H., Chen, S.H., Chuang, A.D.C., and Chen, J.P. (2021). Functional hyaluronic acid-polylactic acid\/silver nanoparticles core-sheath nanofiber membranes for prevention of post-operative tendon adhesion. Int. J. Mol. Sci., 22.","DOI":"10.3390\/ijms22168781"},{"key":"ref_108","doi-asserted-by":"crossref","unstructured":"Grottkau, B.E., Hui, Z., Yao, Y., and Pang, Y. (2020). Rapid Fabrication of Anatomically-Shaped Bone Scaffolds Using Indirect 3D Printing and Perfusion Techniques. Int. J. Mol. Sci., 21.","DOI":"10.3390\/ijms21010315"},{"key":"ref_109","doi-asserted-by":"crossref","first-page":"410","DOI":"10.1177\/03635465020300031701","article-title":"Supplementation of Rotator Cuff Repair with a Bioresorbable Scaffold","volume":"30","author":"Koh","year":"2002","journal-title":"Am. J. Sports Med."},{"key":"ref_110","doi-asserted-by":"crossref","unstructured":"Colonna, M., Zingerle, B., Parisi, M.F., Gioia, C., Speranzoni, A., Pisaneschi, G., and Prosdocimo, S. (2020). A Novel Approach for a Faster Prototyping of Winter Sport Equipment Using Digital Image Correlation and 3D Printing. Proceedings, 49.","DOI":"10.3390\/proceedings2020049125"},{"key":"ref_111","doi-asserted-by":"crossref","first-page":"184","DOI":"10.1016\/j.wasman.2018.11.012","article-title":"How to manage biocomposites wastes end of life? A life cycle assessment approach (LCA) focused on polypropylene (PP)\/wood flour and polylactic acid (PLA)\/flax fibres biocom-posites","volume":"83","author":"Beigbeder","year":"2019","journal-title":"Waste Manag."},{"key":"ref_112","doi-asserted-by":"crossref","first-page":"47132","DOI":"10.1039\/C7RA08869H","article-title":"Complex study of the physical properties of a poly (lactic acid)\/poly (3-hydroxybutyrate) blend and its carbon black composite during various outdoor and laboratory ageing conditions","volume":"7","author":"Danko","year":"2017","journal-title":"RSC Adv."}],"container-title":["Polymers"],"original-title":[],"language":"en","link":[{"URL":"https:\/\/www.mdpi.com\/2073-4360\/15\/14\/3096\/pdf","content-type":"unspecified","content-version":"vor","intended-application":"similarity-checking"}],"deposited":{"date-parts":[[2025,10,10]],"date-time":"2025-10-10T20:15:02Z","timestamp":1760127302000},"score":1,"resource":{"primary":{"URL":"https:\/\/www.mdpi.com\/2073-4360\/15\/14\/3096"}},"subtitle":[],"short-title":[],"issued":{"date-parts":[[2023,7,19]]},"references-count":112,"journal-issue":{"issue":"14","published-online":{"date-parts":[[2023,7]]}},"alternative-id":["polym15143096"],"URL":"https:\/\/doi.org\/10.3390\/polym15143096","relation":{},"ISSN":["2073-4360"],"issn-type":[{"value":"2073-4360","type":"electronic"}],"subject":[],"published":{"date-parts":[[2023,7,19]]}}}