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Among the various directions in OSCs, all-polymer solar cells (all-PSCs) have emerged as a highly promising and currently active research area due to their excellent film formation properties, mechanical properties, and thermal stabilities. However, most of the high-efficiency all-PSCs are processed from chloroform with an active layer thickness of ~100 nm. In order to meet the requirements for industrialization, a thicker active layer processed from low-vapor pressure solvents (preferentially a hydrocarbon solvent) is strongly desired. Herein, we employ toluene (a hydrocarbon solvent with a much higher boiling point than chloroform) and a method known as sequential processing (SqP) to mitigate the rapid decline in efficiency with increasing film thickness. We show that SqP enables a more favorable vertical phase segregation that leads to less trap-assisted recombination and enhanced charge extraction and lifetime than blend-cast devices at higher film thicknesses.<\/jats:p>","DOI":"10.3390\/polym15163462","type":"journal-article","created":{"date-parts":[[2023,8,18]],"date-time":"2023-08-18T10:28:48Z","timestamp":1692354528000},"page":"3462","update-policy":"https:\/\/doi.org\/10.3390\/mdpi_crossmark_policy","source":"Crossref","is-referenced-by-count":4,"title":["All-Polymer Solar Cells Sequentially Solution Processed from Hydrocarbon Solvent with a Thick Active Layer"],"prefix":"10.3390","volume":"15","author":[{"given":"Yajie","family":"Wang","sequence":"first","affiliation":[{"name":"College of New Materials and New Energies, Shenzhen Technology University, Shenzhen 518118, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Chaoyue","family":"Zhao","sequence":"additional","affiliation":[{"name":"College of New Materials and New Energies, Shenzhen Technology University, Shenzhen 518118, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Ziqi","family":"Cai","sequence":"additional","affiliation":[{"name":"Julong College, Shenzhen Technology University, Shenzhen 518118, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Lihong","family":"Wang","sequence":"additional","affiliation":[{"name":"College of New Materials and New Energies, Shenzhen Technology University, Shenzhen 518118, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Liangxiang","family":"Zhu","sequence":"additional","affiliation":[{"name":"College of New Materials and New Energies, Shenzhen Technology University, Shenzhen 518118, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Hui","family":"Huang","sequence":"additional","affiliation":[{"name":"College of New Materials and New Energies, Shenzhen Technology University, Shenzhen 518118, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Guoping","family":"Zhang","sequence":"additional","affiliation":[{"name":"College of New Materials and New Energies, Shenzhen Technology University, Shenzhen 518118, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-0285-7844","authenticated-orcid":false,"given":"Peng","family":"You","sequence":"additional","affiliation":[{"name":"College of New Materials and New Energies, Shenzhen Technology University, Shenzhen 518118, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Chen","family":"Xie","sequence":"additional","affiliation":[{"name":"College of New Materials and New Energies, Shenzhen Technology University, Shenzhen 518118, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Yaping","family":"Wang","sequence":"additional","affiliation":[{"name":"College of New Materials and New Energies, Shenzhen Technology University, Shenzhen 518118, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Qing","family":"Bai","sequence":"additional","affiliation":[{"name":"College of New Materials and New Energies, Shenzhen Technology University, Shenzhen 518118, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Tao","family":"Yang","sequence":"additional","affiliation":[{"name":"Julong College, Shenzhen Technology University, Shenzhen 518118, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"given":"Shunpu","family":"Li","sequence":"additional","affiliation":[{"name":"College of New Materials and New Energies, Shenzhen Technology University, Shenzhen 518118, China"}],"role":[{"role":"author","vocabulary":"crossref"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-2750-7720","authenticated-orcid":false,"given":"Guangye","family":"Zhang","sequence":"additional","affiliation":[{"name":"College of New Materials and New Energies, Shenzhen Technology University, Shenzhen 518118, China"}],"role":[{"role":"author","vocabulary":"crossref"}]}],"member":"1968","published-online":{"date-parts":[[2023,8,18]]},"reference":[{"key":"ref_1","doi-asserted-by":"crossref","first-page":"e2301231","DOI":"10.1002\/adma.202301231","article-title":"Isomeric Solid Additive Enables High-Efficiency Polymer Solar Cells Developed Using a Benzo-difuran-based Donor Polymer","volume":"35","author":"Chen","year":"2023","journal-title":"Adv. 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