{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,6,27]],"date-time":"2026-06-27T00:59:14Z","timestamp":1782521954410,"version":"3.54.5"},"reference-count":64,"publisher":"MDPI AG","issue":"19","license":[{"start":{"date-parts":[[2023,9,26]],"date-time":"2023-09-26T00:00:00Z","timestamp":1695686400000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/creativecommons.org\/licenses\/by\/4.0\/"}],"funder":[{"name":"Pilot research and development of new technology of functional polymer surface protection materials","award":["NBHG2021H0014"],"award-info":[{"award-number":["NBHG2021H0014"]}]},{"name":"Pilot research and development of new technology of functional polymer surface protection materials","award":["52273112"],"award-info":[{"award-number":["52273112"]}]},{"name":"Pilot research and development of new technology of functional polymer surface protection materials","award":["20210322Z0026"],"award-info":[{"award-number":["20210322Z0026"]}]},{"name":"Start-up Funding of National Natural Science Foundation of China","award":["NBHG2021H0014"],"award-info":[{"award-number":["NBHG2021H0014"]}]},{"name":"Start-up Funding of National Natural Science Foundation of China","award":["52273112"],"award-info":[{"award-number":["52273112"]}]},{"name":"Start-up Funding of National Natural Science Foundation of China","award":["20210322Z0026"],"award-info":[{"award-number":["20210322Z0026"]}]},{"name":"Ningbo Research Institute of Zhejiang University","award":["NBHG2021H0014"],"award-info":[{"award-number":["NBHG2021H0014"]}]},{"name":"Ningbo Research Institute of Zhejiang University","award":["52273112"],"award-info":[{"award-number":["52273112"]}]},{"name":"Ningbo Research Institute of Zhejiang University","award":["20210322Z0026"],"award-info":[{"award-number":["20210322Z0026"]}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":["Polymers"],"abstract":"<jats:p>Thermoset powder coatings exhibit distinctive characteristics such as remarkable hardness and exceptional resistance to corrosion. In contrast to conventional paints, powder coatings are environmentally friendly due to the absence of volatile organic compounds (VOCs). However, their irreversible cross-linking structures limit their chain segment mobility, preventing polymers from autonomously repairing cracks. Dynamic cross-linking networks have garnered attention for their remarkable self-healing capabilities, facilitated by rapid internal bond exchange. Herein, we introduce an innovative method for synthesizing thermoset epoxy containing boronic ester moieties which could prolong the life of the powder coating. The epoxy resin system relies on the incorporation of two curing agents: one featuring small-molecule diamines with boronic bonds and the other a modified polyurethane prepolymer. A state of equilibrium in mechanical properties was achieved via precise manipulation of the proportions of these agents, with the epoxy composite exhibiting a fracture stress of 67.95 MPa while maintaining a stable glass transition temperature (Tg) of 51.39 \u00b0C. This imparts remarkable self-healing ability to the coating surface, capable of returning to its original state even after undergoing 1000 cycles of rubbing (using 1200-grit abrasive paper). Furthermore, the introduction of carbon nanotube nanoparticles enabled non-contact sequential self-healing. Subsequently, we introduce this method into powder coatings of different materials. Therefore, this work provides a strategy to develop functional interior decoration and ensure its potential for broad-ranging applications, such as aerospace, transportation, and other fields.<\/jats:p>","DOI":"10.3390\/polym15193894","type":"journal-article","created":{"date-parts":[[2023,9,27]],"date-time":"2023-09-27T03:49:14Z","timestamp":1695786554000},"page":"3894","update-policy":"https:\/\/doi.org\/10.3390\/mdpi_crossmark_policy","source":"Crossref","is-referenced-by-count":8,"title":["A Self-Healing Thermoset Epoxy Modulated by Dynamic Boronic Ester for Powder Coating"],"prefix":"10.3390","volume":"15","author":[{"given":"Yongqi","family":"Liu","sequence":"first","affiliation":[{"name":"Ningbo Research Institute, Zhejiang University, Ningbo 315807, China"},{"name":"State Key Laboratory of Chemical Engineering, College of Chemical and Biological Engineering, Zhejiang University, Hangzhou 310027, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Ziyuan","family":"Li","sequence":"additional","affiliation":[{"name":"School of Biological and Chemical Engineering, Ningbo Tech University, Ningbo 315100, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Caifu","family":"Zhang","sequence":"additional","affiliation":[{"name":"Tongling Shanwei New Material Technology Inc. Co., Ltd., Tongling 244000, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Biru","family":"Yang","sequence":"additional","affiliation":[{"name":"Ningbo Research Institute, Zhejiang University, Ningbo 315807, China"},{"name":"State Key Laboratory of Chemical Engineering, College of Chemical and Biological Engineering, Zhejiang University, Hangzhou 310027, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Hua","family":"Ren","sequence":"additional","affiliation":[{"name":"Ningbo Research Institute, Zhejiang University, Ningbo 315807, China"},{"name":"State Key Laboratory of Chemical Engineering, College of Chemical and Biological Engineering, Zhejiang University, Hangzhou 310027, China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"1968","published-online":{"date-parts":[[2023,9,26]]},"reference":[{"key":"ref_1","doi-asserted-by":"crossref","first-page":"4222","DOI":"10.1016\/j.polymer.2012.07.026","article-title":"Molecular dynamics simulations and experimental studies of the thermomechanical response of an epoxy thermoset polymer","volume":"53","author":"Li","year":"2012","journal-title":"Polymer"},{"key":"ref_2","doi-asserted-by":"crossref","first-page":"35","DOI":"10.1016\/j.compositesa.2014.07.002","article-title":"Prediction of the chemical and thermal shrinkage in a thermoset polymer","volume":"66","author":"Kravchenko","year":"2014","journal-title":"Compos. 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