{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,8,18]],"date-time":"2026-08-18T05:04:10Z","timestamp":1787029450161,"version":"build-2736575974"},"reference-count":51,"publisher":"MDPI AG","issue":"4","license":[{"start":{"date-parts":[[2026,2,11]],"date-time":"2026-02-11T00:00:00Z","timestamp":1770768000000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/creativecommons.org\/licenses\/by\/4.0\/"}],"funder":[{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"crossref","award":["52502047"],"award-info":[{"award-number":["52502047"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"crossref"}]},{"DOI":"10.13039\/501100001809","name":"National Natural Science Foundation of China","doi-asserted-by":"crossref","award":["42030807"],"award-info":[{"award-number":["42030807"]}],"id":[{"id":"10.13039\/501100001809","id-type":"DOI","asserted-by":"crossref"}]},{"DOI":"10.13039\/501100012226","name":"Fundamental Research Funds for the Central Universities","doi-asserted-by":"crossref","award":["2025ZKPYHH02"],"award-info":[{"award-number":["2025ZKPYHH02"]}],"id":[{"id":"10.13039\/501100012226","id-type":"DOI","asserted-by":"crossref"}]},{"name":"Inner Mongolia Autonomous Region Major Science and Technology project","award":["2020ZD0024"],"award-info":[{"award-number":["2020ZD0024"]}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":["Polymers"],"abstract":"<jats:p>The development of smart coatings with active protection is a promising approach to prolonging the service life in extreme environments. Herein, the corrosion inhibitors 2-mercaptobenzimidazole (MBI) and CeO2 were in situ loaded onto the surface of graphene oxide (GO) by dopamine (DA) polymerization, and we ultimately obtained the multifunctional composite MBI@CeO2@PDA@GO (MCPG). The electrochemical impedance spectroscopy (EIS) results revealed that after 30 days of immersion in the corrosive media, the |Z|0.01 Hz value of MCPG\/WEP coating remained at 3.7 \u00d7 109 \u03a9\/cm2, which displayed four orders of magnitude higher than that of pure WEP coating (1.4 \u00d7 105 \u03a9\/cm2). In a 200 h salt spray test, the MCPG\/WEP coating also demonstrated minimal corrosion products and bubbles, affirming the exceptional corrosion-inhibiting effect and excellent self-healing performance. Consequently, the synergistic combination of pH-sensitive properties and outstanding barrier effect imparted dual active\/passive anti-corrosion capabilities to the coating, resulting in long-lasting metal protection.<\/jats:p>","DOI":"10.3390\/polym18040459","type":"journal-article","created":{"date-parts":[[2026,2,11]],"date-time":"2026-02-11T13:25:49Z","timestamp":1770816349000},"page":"459","update-policy":"https:\/\/doi.org\/10.3390\/mdpi_crossmark_policy","source":"Crossref","is-referenced-by-count":1,"title":["PH-Sensitive Self-Healing Waterborne Epoxy Coating: Polydopamine Grafted Graphene Oxide with 2-Mercaptobenzimidazole Inhibitors and Cerium Cation Towards Anti-Corrosion Performance"],"prefix":"10.3390","volume":"18","author":[{"given":"Shengle","family":"Hao","sequence":"first","affiliation":[{"name":"School of Chemical & Environmental Engineering, China University of Mining & Technology (Beijing), Beijing 100083, China"},{"name":"Key Laboratory of Advanced Materials (MOE), School of Materials Science and Engineering, Tsinghua University, Beijing 100084, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Shiyu","family":"Hou","sequence":"additional","affiliation":[{"name":"School of Chemical & Environmental Engineering, China University of Mining & Technology (Beijing), Beijing 100083, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9084-6776","authenticated-orcid":false,"given":"Ding","family":"Nan","sequence":"additional","affiliation":[{"name":"College of Chemistry and Chemical Engineering, Inner Mongolia University, Hohhot 010021, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Deping","family":"Xu","sequence":"additional","affiliation":[{"name":"School of Chemical & Environmental Engineering, China University of Mining & Technology (Beijing), Beijing 100083, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Wanci","family":"Shen","sequence":"additional","affiliation":[{"name":"Key Laboratory of Advanced Materials (MOE), School of Materials Science and Engineering, Tsinghua University, Beijing 100084, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"given":"Feiyu","family":"Kang","sequence":"additional","affiliation":[{"name":"Tsinghua Shenzhen International Graduate School, Tsinghua University, Shenzhen 518055, China"}],"role":[{"vocabulary":"crossref","role":"author"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-0591-6830","authenticated-orcid":false,"given":"Zheng-Hong","family":"Huang","sequence":"additional","affiliation":[{"name":"Key Laboratory of Advanced Materials (MOE), School of Materials Science and Engineering, Tsinghua University, Beijing 100084, China"}],"role":[{"vocabulary":"crossref","role":"author"}]}],"member":"1968","published-online":{"date-parts":[[2026,2,11]]},"reference":[{"key":"ref_1","doi-asserted-by":"crossref","first-page":"159128","DOI":"10.1016\/j.cej.2024.159128","article-title":"A \u201ctwo birds one stone\u201d strategy for self-healing marine coatings with antifouling and anticorrosion properties","volume":"504","author":"Cui","year":"2025","journal-title":"Chem. 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