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(FCT)","award":["UIDP\/00532\/2020"],"award-info":[{"award-number":["UIDP\/00532\/2020"]}]},{"name":"CMAT (Centre of Mathematics of the University of Minho)","award":["PRIN_2022TSLMHR"],"award-info":[{"award-number":["PRIN_2022TSLMHR"]}]},{"name":"CMAT (Centre of Mathematics of the University of Minho)","award":["UIDB\/04650\/2020"],"award-info":[{"award-number":["UIDB\/04650\/2020"]}]},{"name":"CMAT (Centre of Mathematics of the University of Minho)","award":["UIDP\/04650\/2020"],"award-info":[{"award-number":["UIDP\/04650\/2020"]}]},{"name":"CMAT (Centre of Mathematics of the University of Minho)","award":["UIDB\/00013\/2020"],"award-info":[{"award-number":["UIDB\/00013\/2020"]}]},{"name":"CMAT (Centre of Mathematics of the University of Minho)","award":["UIDP\/00013\/2020"],"award-info":[{"award-number":["UIDP\/00013\/2020"]}]},{"name":"CMAT (Centre of Mathematics of the University of Minho)","award":["UIDB\/00532\/2020"],"award-info":[{"award-number":["UIDB\/00532\/2020"]}]},{"name":"CMAT (Centre of Mathematics of the University of Minho)","award":["UIDP\/00532\/2020"],"award-info":[{"award-number":["UIDP\/00532\/2020"]}]},{"name":"CEFT (Transport Phenomena Research Center of the University of Porto)","award":["PRIN_2022TSLMHR"],"award-info":[{"award-number":["PRIN_2022TSLMHR"]}]},{"name":"CEFT (Transport Phenomena Research Center of the University of Porto)","award":["UIDB\/04650\/2020"],"award-info":[{"award-number":["UIDB\/04650\/2020"]}]},{"name":"CEFT (Transport Phenomena Research Center of the University of Porto)","award":["UIDP\/04650\/2020"],"award-info":[{"award-number":["UIDP\/04650\/2020"]}]},{"name":"CEFT (Transport Phenomena Research Center of the University of Porto)","award":["UIDB\/00013\/2020"],"award-info":[{"award-number":["UIDB\/00013\/2020"]}]},{"name":"CEFT (Transport Phenomena Research Center of the University of Porto)","award":["UIDP\/00013\/2020"],"award-info":[{"award-number":["UIDP\/00013\/2020"]}]},{"name":"CEFT (Transport Phenomena Research Center of the University of Porto)","award":["UIDB\/00532\/2020"],"award-info":[{"award-number":["UIDB\/00532\/2020"]}]},{"name":"CEFT (Transport Phenomena Research Center of the University of Porto)","award":["UIDP\/00532\/2020"],"award-info":[{"award-number":["UIDP\/00532\/2020"]}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":["Gels"],"abstract":"<jats:p>Self-assembled peptide-based hydrogels have attracted considerable interest from the research community. Particularly, low molecular weight gelators (LMWGs) consisting of amino acids and short peptides are highly suitable for biological applications owing to their facile synthesis and scalability, as well as their biocompatibility, biodegradability, and stability in physiological conditions. However, challenges in understanding the structure\u2013property relationship and lack of design rules hinder the development of new gelators with the required properties for several applications. Hereby, in the plethora of peptide-based gelators, this review discusses the mechanical properties of single amino acid and dipeptide-based hydrogels. A mutual analysis of these systems allows us to highlight the relationship between the gel mechanical properties and amino acid sequence, preparation methods, or N capping groups. Additionally, recent advancements in the tuning of the gels\u2019 rheological properties are reviewed. In this way, the present review aims to help bridge the knowledge gap between structure and mechanical properties, easing the selection or design of peptides with the required properties for biological applications.<\/jats:p>","DOI":"10.3390\/gels10080507","type":"journal-article","created":{"date-parts":[[2024,8,1]],"date-time":"2024-08-01T12:38:20Z","timestamp":1722515900000},"page":"507","update-policy":"https:\/\/doi.org\/10.3390\/mdpi_crossmark_policy","source":"Crossref","is-referenced-by-count":14,"title":["A Review on the Rheological Properties of Single Amino Acids and Short Dipeptide Gels"],"prefix":"10.3390","volume":"10","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-2724-5772","authenticated-orcid":false,"given":"S\u00e9rgio R. S.","family":"Veloso","sequence":"first","affiliation":[{"name":"Physics Centre of Minho and Porto Universities (CF-UM-UP), Laboratory of Physics for Materials and Emergent Technologies (LaPMET), University of Minho, Campus of Gualtar, 4710-057 Braga, Portugal"}]},{"given":"Mariangela","family":"Rosa","sequence":"additional","affiliation":[{"name":"Department of Pharmacy, Centro Interuniversitario di Ricerca sui Peptidi Bioattivi \u201cCarlo Pedone\u201d (CIRPeB), University of Naples \u201cFederico II\u201d, Via Tommaso de Amicis 95, 80131 Naples, Italy"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-9273-0136","authenticated-orcid":false,"given":"Carlo","family":"Diaferia","sequence":"additional","affiliation":[{"name":"Department of Pharmacy, Centro Interuniversitario di Ricerca sui Peptidi Bioattivi \u201cCarlo Pedone\u201d (CIRPeB), University of Naples \u201cFederico II\u201d, Via Tommaso de Amicis 95, 80131 Naples, Italy"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-0340-3556","authenticated-orcid":false,"given":"C\u00e9lio","family":"Fernandes","sequence":"additional","affiliation":[{"name":"Transport Phenomena Research Centre (CEFT), Department of Mechanical Engineering, Faculty of Engineering, University of Porto (FEUP), Rua Dr. Roberto Frias s\/n, 4200-465 Porto, Portugal"},{"name":"Centre of Mathematics (CMAT), School of Sciences, University of Minho, Campus of Gualtar, 4710-057 Braga, Portugal"}]}],"member":"1968","published-online":{"date-parts":[[2024,8,1]]},"reference":[{"key":"ref_1","doi-asserted-by":"crossref","first-page":"482","DOI":"10.1016\/j.addr.2021.05.010","article-title":"Peptide-Based Supramolecular Hydrogels for Local Drug Delivery","volume":"174","author":"Zhang","year":"2021","journal-title":"Adv. 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