{"status":"ok","message-type":"work","message-version":"1.0.0","message":{"indexed":{"date-parts":[[2026,3,28]],"date-time":"2026-03-28T10:37:58Z","timestamp":1774694278300,"version":"3.50.1"},"reference-count":210,"publisher":"MDPI AG","issue":"10","license":[{"start":{"date-parts":[[2023,5,21]],"date-time":"2023-05-21T00:00:00Z","timestamp":1684627200000},"content-version":"vor","delay-in-days":0,"URL":"https:\/\/creativecommons.org\/licenses\/by\/4.0\/"}],"funder":[{"DOI":"10.13039\/501100004359","name":"Swedish Research Council","doi-asserted-by":"publisher","award":["2022-04425"],"award-info":[{"award-number":["2022-04425"]}],"id":[{"id":"10.13039\/501100004359","id-type":"DOI","asserted-by":"publisher"}]}],"content-domain":{"domain":[],"crossmark-restriction":false},"short-container-title":["Molecules"],"abstract":"<jats:p>In the history of cellulose chemistry, hydrogen bonding has been the predominant explanation when discussing intermolecular interactions between cellulose polymers. This is the general consensus in scholarly textbooks and in many research articles, and it applies to several other biomacromolecules\u2019 interactions as well. This rather unbalanced description of cellulose has likely impacted the development of materials based on the processing of cellulose\u2014for example, via dissolution in various solvent systems and regeneration into solid materials, such as films and fibers, and even traditional wood fiber handling and papermaking. In this review, we take as a starting point the questioning of the general description of the nature of cellulose and cellulose interactions initiated by Professor Bj\u00f6rn Lindman, based on generic physicochemical reasoning about surfactants and polymers. This dispute, which became known as \u201cthe Lindman hypothesis\u201d, highlights the importance of hydrophobic interactions in cellulose systems and that cellulose is an amphiphilic polymer. This paper elaborates on Bj\u00f6rn Lindman\u2019s contribution to the subject, which has caused the scientific community to revisit cellulose and reconsider certain phenomena from other perspectives.<\/jats:p>","DOI":"10.3390\/molecules28104216","type":"journal-article","created":{"date-parts":[[2023,5,22]],"date-time":"2023-05-22T02:00:27Z","timestamp":1684720827000},"page":"4216","update-policy":"https:\/\/doi.org\/10.3390\/mdpi_crossmark_policy","source":"Crossref","is-referenced-by-count":27,"title":["Perspectives on the Lindman Hypothesis and Cellulose Interactions"],"prefix":"10.3390","volume":"28","author":[{"ORCID":"https:\/\/orcid.org\/0000-0003-3407-7973","authenticated-orcid":false,"given":"Magnus","family":"Norgren","sequence":"first","affiliation":[{"name":"Surface and Colloid Engineering, FSCN Research Centre, Mid Sweden University, SE-851 70 Sundsvall, Sweden"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-8223-4166","authenticated-orcid":false,"given":"Carolina","family":"Costa","sequence":"additional","affiliation":[{"name":"Surface and Colloid Engineering, FSCN Research Centre, Mid Sweden University, SE-851 70 Sundsvall, Sweden"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-4447-5107","authenticated-orcid":false,"given":"Lu\u00eds","family":"Alves","sequence":"additional","affiliation":[{"name":"Department of Chemical Engineering, CIEPQPF\u2014Chemical Processes and Forest Products Engineering Research Centre, University of Coimbra, P\u00f3lo II\u2013R. Silvio Lima, 3030-790 Coimbra, Portugal"}]},{"ORCID":"https:\/\/orcid.org\/0000-0001-6270-2970","authenticated-orcid":false,"given":"Alireza","family":"Eivazi","sequence":"additional","affiliation":[{"name":"Surface and Colloid Engineering, FSCN Research Centre, Mid Sweden University, SE-851 70 Sundsvall, Sweden"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-3439-0505","authenticated-orcid":false,"given":"Christina","family":"Dahlstr\u00f6m","sequence":"additional","affiliation":[{"name":"Surface and Colloid Engineering, FSCN Research Centre, Mid Sweden University, SE-851 70 Sundsvall, Sweden"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-1670-6783","authenticated-orcid":false,"given":"Ida","family":"Svanedal","sequence":"additional","affiliation":[{"name":"Surface and Colloid Engineering, FSCN Research Centre, Mid Sweden University, SE-851 70 Sundsvall, Sweden"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-5579-3373","authenticated-orcid":false,"given":"H\u00e5kan","family":"Edlund","sequence":"additional","affiliation":[{"name":"Surface and Colloid Engineering, FSCN Research Centre, Mid Sweden University, SE-851 70 Sundsvall, Sweden"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-0972-1739","authenticated-orcid":false,"given":"Bruno","family":"Medronho","sequence":"additional","affiliation":[{"name":"Surface and Colloid Engineering, FSCN Research Centre, Mid Sweden University, SE-851 70 Sundsvall, Sweden"},{"name":"MED\u2014Mediterranean Institute for Agriculture, Environment and Development, CHANGE\u2014Global Change and Sustainability Institute, Faculdade de Ci\u00eancias e Tecnologia, Universidade do Algarve, Campus de Gambelas, Ed. 8, 8005-139 Faro, Portugal"}]}],"member":"1968","published-online":{"date-parts":[[2023,5,21]]},"reference":[{"key":"ref_1","doi-asserted-by":"crossref","first-page":"76","DOI":"10.1016\/j.molliq.2010.04.016","article-title":"On the Mechanism of Dissolution of Cellulose","volume":"156","author":"Lindman","year":"2010","journal-title":"J. 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