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They can be synthesized with specific features to be used as adsorbents, resulting in improved performance for wastewater pollutants\u2019 removal. The purpose of this research was to investigate the effect of amino functionalization and the addition of carbon nanostructures to silica aerogels made from methyltrimethoxysilane (MTMS) on their removal capacities for various contaminants in aqueous solutions. The MTMS-based aerogels successfully removed various organic compounds and drugs, achieving adsorption capacities of 170 mg\u22c5g\u22121 for toluene and 200 mg\u22c5g\u22121 for xylene. For initial concentrations up to 50 mg\u22c5L\u22121, removals greater than 71% were obtained for amoxicillin, and superior to 96% for naproxen. The addition of a co-precursor containing amine groups and\/or carbon nanomaterials was proven to be a valuable tool in the development of new adsorbents by altering the aerogels\u2019 properties and enhancing their adsorption capacities. Therefore, this work demonstrates the potential of these materials as an alternative to industrial sorbents due to their high and fast removal efficiency, less than 60 min for the organic compounds, towards different types of pollutants.<\/jats:p>","DOI":"10.3390\/toxics11030232","type":"journal-article","created":{"date-parts":[[2023,2,28]],"date-time":"2023-02-28T02:01:51Z","timestamp":1677549711000},"page":"232","update-policy":"https:\/\/doi.org\/10.3390\/mdpi_crossmark_policy","source":"Crossref","is-referenced-by-count":22,"title":["Carbon Nanostructures\u2014Silica Aerogel Composites for Adsorption of Organic Pollutants"],"prefix":"10.3390","volume":"11","author":[{"ORCID":"https:\/\/orcid.org\/0000-0002-5948-0921","authenticated-orcid":false,"given":"Alyne","family":"Lamy-Mendes","sequence":"first","affiliation":[{"name":"University of Coimbra, CIEPQPF\u2014Chemical Process Engineering and Forest Products Research Centre, Department of Chemical Engineering, 3030-790 Coimbra, Portugal"},{"name":"CICECO\u2014Aveiro Institute of Materials, Department of Materials and Ceramic Engineering, University of Aveiro, 3810-193 Aveiro, Portugal"}]},{"given":"David","family":"Lopes","sequence":"additional","affiliation":[{"name":"University of Coimbra, CIEPQPF\u2014Chemical Process Engineering and Forest Products Research Centre, Department of Chemical Engineering, 3030-790 Coimbra, Portugal"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-2699-646X","authenticated-orcid":false,"given":"Ana V.","family":"Gir\u00e3o","sequence":"additional","affiliation":[{"name":"CICECO\u2014Aveiro Institute of Materials, Department of Materials and Ceramic Engineering, University of Aveiro, 3810-193 Aveiro, Portugal"}]},{"ORCID":"https:\/\/orcid.org\/0000-0002-2584-1792","authenticated-orcid":false,"given":"Rui F.","family":"Silva","sequence":"additional","affiliation":[{"name":"CICECO\u2014Aveiro Institute of Materials, Department of Materials and Ceramic Engineering, University of Aveiro, 3810-193 Aveiro, Portugal"}]},{"given":"Wim J.","family":"Malfait","sequence":"additional","affiliation":[{"name":"Laboratory for Building Energy Materials and Components, Empa\u2014Swiss Federal Laboratory for Science and Technology, \u00dcberlandstrasse 129, 8600 D\u00fcbendorf, Switzerland"}]},{"ORCID":"https:\/\/orcid.org\/0000-0003-3336-2449","authenticated-orcid":false,"given":"Lu\u00edsa","family":"Dur\u00e3es","sequence":"additional","affiliation":[{"name":"University of Coimbra, CIEPQPF\u2014Chemical Process Engineering and Forest Products Research Centre, Department of Chemical Engineering, 3030-790 Coimbra, Portugal"}]}],"member":"1968","published-online":{"date-parts":[[2023,2,28]]},"reference":[{"key":"ref_1","doi-asserted-by":"crossref","first-page":"173","DOI":"10.1016\/j.cej.2018.05.189","article-title":"Compressive, Ultralight and Fire-Resistant Lignin-Modified Graphene Aerogels as Recyclable Absorbents for Oil and Organic Solvents","volume":"350","author":"Chen","year":"2018","journal-title":"Chem. 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